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In this work, a series of N\u2010doped porous carbons (PDA@HCP(x:y)\u2010T) was prepared; the CO<jats:sub>2<\/jats:sub> adsorption capacity of the prepared PDA@HCP(x:y)\u2010T was enhanced by coating polydopamine (PDA) on a hypercross\u2010linked polymer (HCP) and then adjusting the mass ratio of PDA to HCP and the carbonization temperature. The results showed that the prepared PDA@HCP(1\u2009:\u20091)\u2010850 exhibited a high CO<jats:sub>2<\/jats:sub> adsorption capacity due to abundant micropores (0.6762\u2005cm<jats:sup>3<\/jats:sup>\/g), a high specific surface area (1220.8\u2005m<jats:sup>2<\/jats:sup>\/g), and moderate surface nitrogen content (2.75\u2009%). Notably, PDA@HCP(1\u2009:\u20091)\u2010850 exhibited the highest CO<jats:sub>2<\/jats:sub> uptake of 6.46\u2005mmol\/g at 0\u2009\u00b0C and 101\u2005kPa. Critically, these N\u2010doped porous carbons can also be used as catalysts for the reaction of CO<jats:sub>2<\/jats:sub> with epichlorohydrin to form chloropropylene carbonate, with chloropropylene carbonate yielding up to 64\u2009% and selectivity of the reaction reaching 94\u2009%. As a result, these N\u2010doped porous carbons could serve as potential candidates for CO<jats:sub>2<\/jats:sub> capture and conversion due to their high reactivity, excellent CO<jats:sub>2<\/jats:sub> uptake, and good catalytic performance.<\/jats:p>","DOI":"10.1002\/chem.202402855","type":"journal-article","created":{"date-parts":[[2024,10,8]],"date-time":"2024-10-08T00:40:11Z","timestamp":1728348011000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":10,"title":["N\u2010doped Porous Carbon Derived from the Pyrolysis of a Polydopamine\u2010coated Hypercross\u2010linked Polymer for Enhanced CO<sub>2<\/sub> Adsorption"],"prefix":"10.1002","volume":"30","author":[{"given":"Jingtao","family":"Wang","sequence":"first","affiliation":[{"name":"College of Chemical Engineering Nanjing Tech University  Nanjing 211816 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xiaoyan","family":"Liu","sequence":"additional","affiliation":[{"name":"College of Chemical Engineering Nanjing Tech University  Nanjing 211816 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yang","family":"Zhou","sequence":"additional","affiliation":[{"name":"College of Chemical Engineering Nanjing Tech University  Nanjing 211816 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-0667-9176","authenticated-orcid":false,"given":"Zhuhong","family":"Yang","sequence":"additional","affiliation":[{"name":"College of Chemical Engineering Nanjing Tech University  Nanjing 211816 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Isaac D.","family":"Tegladza","sequence":"additional","affiliation":[{"name":"College of Chemical Engineering Nanjing Tech University  Nanjing 211816 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Chang","family":"Liu","sequence":"additional","affiliation":[{"name":"College of Chemical Engineering Nanjing Tech University  Nanjing 211816 China"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2024,11,6]]},"reference":[{"key":"e_1_2_8_1_1","unstructured":"\u00a0"},{"key":"e_1_2_8_2_2","unstructured":"G.\u2005M. 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