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Yet, it remains unclear whether this unique weak interaction can induce chirality or not. Herein, we report the synthesis of chiral carbon\u2010bonding donors, and present the proof\u2010of\u2010concept study on asymmetric induction using this noncovalent force. Employing the oxa\u2010Pictet\u2013Spengler reaction as a benchmark, the experimental results demonstrate that chiral carbon\u2010bonding donors can exert asymmetric induction over oxocarbenium ion intermediates. While the enantioselectivity in such a very first attempt is modest, it unequivocally validates carbon bonding as a feasible method for asymmetric induction, paving the way for its future development in more efficient asymmetric synthesis.<\/jats:p>","DOI":"10.1002\/chem.70827","type":"journal-article","created":{"date-parts":[[2026,3,8]],"date-time":"2026-03-08T21:25:46Z","timestamp":1773005146000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Asymmetric Induction With Chiral Carbon\u2010Bonding Donors"],"prefix":"10.1002","volume":"32","author":[{"given":"Yuanling","family":"Pang","sequence":"first","affiliation":[{"name":"School of Chemistry and Chemical Engineering Shandong University  Jinan China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xinxin","family":"Li","sequence":"additional","affiliation":[{"name":"School of Chemistry and Chemical Engineering Shandong University  Jinan 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