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This review surveys recent progress in extending PISA to nonlinear polymers\u2014highlighting how polymer topology reshapes nucleation, packing, interfacial curvature, and ultimately nanoparticle morphology\u2014while also positioning PISA as a practical method for synthesizing architecturally complex macromolecules. Key advances are summarized across star, graft, bottlebrush, branched, and cyclic polymers. 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