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Cleavage of these linkages under catalytic conditions, however, can compromise structural definition and control at the interface. Here, we introduce a ligand\u2010encoded anchoring strategy in which a platinum(II) bis(NHC) complex is immobilized on mesoporous silica (SBA\u201015) exclusively through directional, non\u2010covalent F\u2013Si interactions. The molecular pre\u2010catalyst\n                    <jats:italic>trans<\/jats:italic>\n                    \u2010[Pt(L\n                    <jats:sup>F<\/jats:sup>\n                    )\n                    <jats:sub>2<\/jats:sub>\n                    Cl\n                    <jats:sub>2<\/jats:sub>\n                    ] was structurally characterized by single\u2010crystal X\u2010ray diffraction and multinuclear solution\u2010state NMR spectroscopy. Advanced solid\u2010state MAS NMR experiments, including\n                    <jats:sup>19<\/jats:sup>\n                    F{\n                    <jats:sup>29<\/jats:sup>\n                    Si} REDOR, combined with molecular dynamics simulations, establish well\u2010defined F\u2013Si contacts with internuclear distances on the \u00c5\u2010scale and reveal the organization of the pre\u2010catalyst at the silica interface. A model hydrosilylation reaction demonstrates catalytic activity and retention of the molecular species on the support during turnover. This work establishes non\u2010covalent interface engineering as a viable strategy for structurally defined heterogenized catalysis.\n                  <\/jats:p>","DOI":"10.1002\/chem.71585","type":"journal-article","created":{"date-parts":[[2026,9,1]],"date-time":"2026-09-01T10:14:49Z","timestamp":1788257689000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Non\u2010Covalent Fluorine\u2013Silica Anchoring of a Molecular Platinum(II) bis(NHC) Catalyst: Structure, Interface Control, and Hydrosilylation Activity"],"prefix":"10.1002","author":[{"ORCID":"https:\/\/orcid.org\/0000-0002-3453-8197","authenticated-orcid":false,"given":"Alexander","family":"Bergen","sequence":"first","affiliation":[{"name":"Department of Chemistry and Pharmacy, Inorganic Chemistry Friedrich\u2010Alexander\u2010Universit\u00e4t Erlangen\u2010N\u00fcrnberg (FAU) Erlangen 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