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Their core advantage lies in the ability to precisely control energy levels and safety through molecular\u2010level design. However, the inherent contradiction between high energy and high safety is a key bottleneck restricting their development. This article systematically reviews the crystallographic and physicochemical origins of the contradiction between energy and safety in PEMs, and delves into the research progress on balancing this contradiction through two major strategies: internal crystal engineering (such as component design and intermolecular interaction regulation) and synergistic use of exogenous components (such as composites with metal\/metal oxides, polymer coating technology, and composites with high\u2010energy inductive explosives). Finally, based on the existing foundation, the article looks forward to the opportunities and challenges facing PEMs in terms of deepening mechanism research, expanding multifunctionality, and industrial applications.\n                  <\/jats:p>","DOI":"10.1002\/chem.71616","type":"journal-article","created":{"date-parts":[[2026,9,23]],"date-time":"2026-09-23T11:26:01Z","timestamp":1790162761000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Towards a Balance between Functionality and Stability: Energy\u2010Safety Synergistic Mechanisms and Prospects in Perovskite Energetic Materials"],"prefix":"10.1002","author":[{"ORCID":"https:\/\/orcid.org\/0009-0009-7879-0229","authenticated-orcid":false,"given":"Hongbo","family":"Liang","sequence":"first","affiliation":[{"name":"State Key Laboratory of Explosion Science and Safety Protection Beijing Institute of Technology  Beijing 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