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Most importantly, we show how a sum over intensities for a select region of detection wavelengths and Fourier transform of data over select temporal window untwine contributions from vibrational modes of different origins. Thus, in a single pump\u2010probe experiment, vibrational features specific to solute as well as solvent are disentangled that are otherwise spectrally overlapping and are non\u2010separable in conventional (spontaneous\/stimulated) Raman spectroscopy employing narrowband excitation. We envision wide\u2010ranging applications of this method to unveil vibrational features in complex molecular systems.<\/jats:p>","DOI":"10.1002\/cphc.202300087","type":"journal-article","created":{"date-parts":[[2023,5,26]],"date-time":"2023-05-26T05:22:50Z","timestamp":1685078570000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":5,"title":["Separating Vibrational Coherences in Ground\/Excited Electronic States of Solvent\/Solute Following Non\u2010Resonant\/Resonant Impulsive Excitation"],"prefix":"10.1002","volume":"24","author":[{"given":"Shaina","family":"Dhamija","sequence":"first","affiliation":[{"name":"Condensed Phase Dynamics Group, Department of Chemical Sciences Indian Institute of Science Education and Research Mohali, Knowledge City, Sector 81, SAS Nagar  Punjab 140306 India"},{"name":"Present address: Department of Molecular Spectroscopy Max Planck Institute for Polymer Research  Ackermannweg 10 55128 Mainz 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