{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,4,27]],"date-time":"2026-04-27T07:39:49Z","timestamp":1777275589291,"version":"3.51.4"},"reference-count":80,"publisher":"Wiley","issue":"7","license":[{"start":{"date-parts":[[2026,4,9]],"date-time":"2026-04-09T00:00:00Z","timestamp":1775692800000},"content-version":"vor","delay-in-days":0,"URL":"http:\/\/onlinelibrary.wiley.com\/termsAndConditions#vor"},{"start":{"date-parts":[[2026,4,9]],"date-time":"2026-04-09T00:00:00Z","timestamp":1775692800000},"content-version":"tdm","delay-in-days":0,"URL":"http:\/\/doi.wiley.com\/10.1002\/tdm_license_1.1"}],"funder":[{"DOI":"10.13039\/501100021171","name":"Guangdong Basic and Applied Basic Research Foundation","doi-asserted-by":"publisher","award":["2025A1515012077"],"award-info":[{"award-number":["2025A1515012077"]}],"id":[{"id":"10.13039\/501100021171","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100011492","name":"Jiangmen Science and Technology Bureau","doi-asserted-by":"publisher","award":["2320002001062"],"award-info":[{"award-number":["2320002001062"]}],"id":[{"id":"10.13039\/501100011492","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":["chemistry-europe.onlinelibrary.wiley.com"],"crossmark-restriction":true},"short-container-title":["ChemPhysChem"],"published-print":{"date-parts":[[2026,4,14]]},"abstract":"<jats:p>Liquid\u2010phase shear exfoliation (LPSE) is an efficient and scalable technique for the exfoliation of layered materials. By harnessing fluid shear forces to overcome interlayer van der Waals interactions, LPSE enables the preparation of two\u2010dimensional materials such as graphene, transition metal dichalcogenides, hexagonal boron nitride, and so on. This method offers several advantages, including operational simplicity, high yield, low defect density, and environmental compatibility. In recent years, substantial breakthroughs have been achieved in mechanism understanding, process optimization, and application development. With a focus on graphene as a representative system, this review summarizes recent advances in the energy pathways, mechanisms of LPSE of layered materials, and strategies for optimizing energy utilization in LPSE. Particular emphasis is placed on the processes of energy transfer and transformation during shear\u2010induced exfoliation, aiming to deepen the understanding of energy pathways and to guide the future development of shear exfoliation technology from the perspective of energy pathway regulation.<\/jats:p>","DOI":"10.1002\/cphc.202500807","type":"journal-article","created":{"date-parts":[[2026,4,10]],"date-time":"2026-04-10T05:11:46Z","timestamp":1775797906000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Advances in the Investigation of Energy Pathways During Liquid\u2010Phase Shear Exfoliation of Layered Materials"],"prefix":"10.1002","volume":"27","author":[{"given":"Mingcheng","family":"Mo","sequence":"first","affiliation":[{"name":"Shanghai Key Laboratory of Materials Protection and Advanced Materials in Electric Power Shanghai University of Electric Power  Shanghai China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Jianfeng","family":"Mao","sequence":"additional","affiliation":[{"name":"School of Chemical Engineering The University of Adelaide  Adelaide South Australia Australia"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Jun","family":"Wang","sequence":"additional","affiliation":[{"name":"Key Laboratory for Liquid\u2010Solid Structural Evolution and Processing of Materials (Ministry of Education) Shandong University  Jinan China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-7910-9436","authenticated-orcid":false,"given":"Yajie","family":"Liu","sequence":"additional","affiliation":[{"name":"Advanced Energy Storage Materials and Technology Research Center Guangdong\u2010Hong Kong Joint Laboratory for Carbon Neutrality Jiangmen Laboratory of Carbon Science and Technology  Jiangmen China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-9784-7536","authenticated-orcid":false,"given":"Zhixin","family":"Tai","sequence":"additional","affiliation":[{"name":"Advanced Energy Storage Materials and Technology Research Center Guangdong\u2010Hong Kong Joint Laboratory for Carbon Neutrality Jiangmen Laboratory of Carbon Science and Technology  Jiangmen China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-2485-9509","authenticated-orcid":false,"given":"Baofeng","family":"Wang","sequence":"additional","affiliation":[{"name":"Shanghai Key Laboratory of Materials Protection and Advanced Materials in Electric Power Shanghai University of Electric Power  Shanghai China"}],"role":[{"role":"author","vocabulary":"crossref"}]}],"member":"311","published-online":{"date-parts":[[2026,4,9]]},"reference":[{"key":"e_1_2_9_2_1","doi-asserted-by":"publisher","DOI":"10.1126\/science.1102896"},{"key":"e_1_2_9_3_1","doi-asserted-by":"publisher","DOI":"10.1038\/nmat3944"},{"key":"e_1_2_9_4_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.ceramint.2015.04.143"},{"key":"e_1_2_9_5_1","doi-asserted-by":"publisher","DOI":"10.1021\/cm5044864"},{"key":"e_1_2_9_6_1","doi-asserted-by":"publisher","DOI":"10.1088\/2053-1583\/aae7e3"},{"key":"e_1_2_9_7_1","doi-asserted-by":"publisher","DOI":"10.1007\/s40820-021-00617-3"},{"key":"e_1_2_9_8_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.cej.2023.147551"},{"key":"e_1_2_9_9_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.mattod.2025.03.026"},{"key":"e_1_2_9_10_1","doi-asserted-by":"publisher","DOI":"10.1007\/s10853-017-1049-y"},{"key":"e_1_2_9_11_1","doi-asserted-by":"publisher","DOI":"10.1002\/adfm.202400341"},{"key":"e_1_2_9_12_1","doi-asserted-by":"publisher","DOI":"10.1038\/nnano.2008.215"},{"key":"e_1_2_9_13_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.cemconres.2025.107881"},{"key":"e_1_2_9_14_1","first-page":"51955","article-title":"Exfoliated Nanographite Inorganic\u2010Based Composite Using Microfluidization","volume":"10","author":"Ciriaco D. M.","year":"2025","journal-title":"ACS Omega"},{"key":"e_1_2_9_15_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41598-025-85552-8"},{"key":"e_1_2_9_16_1","doi-asserted-by":"publisher","DOI":"10.3390\/foods14213717"},{"key":"e_1_2_9_17_1","doi-asserted-by":"publisher","DOI":"10.1039\/D3RA07342D"},{"key":"e_1_2_9_18_1","doi-asserted-by":"publisher","DOI":"10.1002\/bkcs.12807"},{"key":"e_1_2_9_19_1","doi-asserted-by":"publisher","DOI":"10.3390\/nano8110942"},{"key":"e_1_2_9_20_1","doi-asserted-by":"publisher","DOI":"10.1063\/5.0090717"},{"key":"e_1_2_9_21_1","doi-asserted-by":"publisher","DOI":"10.1007\/s11051-024-06062-8"},{"key":"e_1_2_9_22_1","doi-asserted-by":"publisher","DOI":"10.1002\/aocs.12900"},{"key":"e_1_2_9_23_1","doi-asserted-by":"publisher","DOI":"10.1002\/adma.202310999"},{"key":"e_1_2_9_24_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.compositesa.2022.106886"},{"key":"e_1_2_9_25_1","doi-asserted-by":"publisher","DOI":"10.1002\/aenm.201803210"},{"key":"e_1_2_9_26_1","doi-asserted-by":"publisher","DOI":"10.1002\/adma.201700605"},{"key":"e_1_2_9_27_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.carbon.2014.07.035"},{"key":"e_1_2_9_28_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.wear.2009.12.036"},{"key":"e_1_2_9_29_1","doi-asserted-by":"publisher","DOI":"10.1039\/C4RA05635C"},{"key":"e_1_2_9_30_1","doi-asserted-by":"publisher","DOI":"10.1021\/acs.langmuir.5c02005"},{"key":"e_1_2_9_31_1","doi-asserted-by":"publisher","DOI":"10.1007\/s10853-023-08897-3"},{"key":"e_1_2_9_32_1","doi-asserted-by":"publisher","DOI":"10.1039\/C6RA15310K"},{"key":"e_1_2_9_33_1","doi-asserted-by":"publisher","DOI":"10.1557\/adv.2019.13"},{"key":"e_1_2_9_34_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.cej.2023.148263"},{"key":"e_1_2_9_35_1","doi-asserted-by":"publisher","DOI":"10.1039\/C4NR03560G"},{"key":"e_1_2_9_36_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.molliq.2023.121848"},{"key":"e_1_2_9_37_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41467-018-05786-1"},{"key":"e_1_2_9_38_1","doi-asserted-by":"publisher","DOI":"10.1063\/5.0170175"},{"key":"e_1_2_9_39_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.energy.2024.130475"},{"key":"e_1_2_9_40_1","doi-asserted-by":"publisher","DOI":"10.1002\/adma.201705791"},{"key":"e_1_2_9_41_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.ultsonch.2018.02.028"},{"key":"e_1_2_9_42_1","doi-asserted-by":"publisher","DOI":"10.1039\/C4RA01250J"},{"key":"e_1_2_9_43_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41598-018-35008-z"},{"key":"e_1_2_9_44_1","doi-asserted-by":"publisher","DOI":"10.1088\/1361-6528\/ac2096"},{"key":"e_1_2_9_45_1","doi-asserted-by":"publisher","DOI":"10.1017\/jfm.2019.938"},{"key":"e_1_2_9_46_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.ultsonch.2020.105214"},{"key":"e_1_2_9_47_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.mineng.2019.106137"},{"key":"e_1_2_9_48_1","doi-asserted-by":"publisher","DOI":"10.1021\/acs.nanolett.4c04329"},{"key":"e_1_2_9_49_1","doi-asserted-by":"publisher","DOI":"10.1016\/S1872-5805(18)60351-8"},{"key":"e_1_2_9_50_1","doi-asserted-by":"publisher","DOI":"10.1017\/jfm.2016.281"},{"key":"e_1_2_9_51_1","doi-asserted-by":"publisher","DOI":"10.1021\/acs.chemmater.6b03335"},{"key":"e_1_2_9_52_1","doi-asserted-by":"publisher","DOI":"10.1088\/1361-6528\/abef2d"},{"key":"e_1_2_9_53_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.jmat.2021.03.007"},{"key":"e_1_2_9_54_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41467-024-55131-y"},{"key":"e_1_2_9_55_1","doi-asserted-by":"publisher","DOI":"10.1021\/acs.chemmater.7b02752"},{"key":"e_1_2_9_56_1","doi-asserted-by":"publisher","DOI":"10.1021\/acs.iecr.0c01744"},{"key":"e_1_2_9_57_1","doi-asserted-by":"publisher","DOI":"10.1021\/acsanm.3c02359"},{"key":"e_1_2_9_58_1","doi-asserted-by":"publisher","DOI":"10.1002\/advs.202417576"},{"key":"e_1_2_9_59_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.ces.2024.119742"},{"key":"e_1_2_9_60_1","doi-asserted-by":"publisher","DOI":"10.1088\/2053-1583\/abdf2f"},{"key":"e_1_2_9_61_1","doi-asserted-by":"publisher","DOI":"10.1021\/acs.iecr.8b01726"},{"key":"e_1_2_9_62_1","doi-asserted-by":"publisher","DOI":"10.1021\/acs.langmuir.0c02517"},{"key":"e_1_2_9_63_1","doi-asserted-by":"publisher","DOI":"10.1021\/ar300009f"},{"key":"e_1_2_9_64_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.jiec.2024.06.028"},{"key":"e_1_2_9_65_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.carbon.2016.02.046"},{"key":"e_1_2_9_66_1","doi-asserted-by":"publisher","DOI":"10.1039\/D3NA00737E"},{"key":"e_1_2_9_67_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.cherd.2008.12.011"},{"key":"e_1_2_9_68_1","doi-asserted-by":"publisher","DOI":"10.1111\/jfpe.70194"},{"key":"e_1_2_9_69_1","doi-asserted-by":"publisher","DOI":"10.3390\/cryst9080377"},{"key":"e_1_2_9_70_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.ces.2021.117132"},{"key":"e_1_2_9_71_1","doi-asserted-by":"publisher","DOI":"10.1039\/D5TA00740B"},{"key":"e_1_2_9_72_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.supflu.2021.105496"},{"key":"e_1_2_9_73_1","doi-asserted-by":"publisher","DOI":"10.1039\/C9RA02102G"},{"key":"e_1_2_9_74_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.jece.2023.109350"},{"key":"e_1_2_9_75_1","doi-asserted-by":"publisher","DOI":"10.1039\/D1TA07915H"},{"key":"e_1_2_9_76_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.jallcom.2024.174214"},{"key":"e_1_2_9_77_1","doi-asserted-by":"publisher","DOI":"10.3390\/nano11030601"},{"key":"e_1_2_9_78_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.cej.2022.138365"},{"key":"e_1_2_9_79_1","doi-asserted-by":"publisher","DOI":"10.1021\/acs.iecr.7b04087"},{"key":"e_1_2_9_80_1","doi-asserted-by":"publisher","DOI":"10.1007\/s13738-025-03180-5"},{"key":"e_1_2_9_81_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.ces.2021.116848"}],"container-title":["ChemPhysChem"],"original-title":[],"language":"en","link":[{"URL":"https:\/\/chemistry-europe.onlinelibrary.wiley.com\/doi\/pdf\/10.1002\/cphc.202500807","content-type":"application\/pdf","content-version":"vor","intended-application":"text-mining"},{"URL":"https:\/\/chemistry-europe.onlinelibrary.wiley.com\/doi\/full-xml\/10.1002\/cphc.202500807","content-type":"application\/xml","content-version":"vor","intended-application":"text-mining"},{"URL":"https:\/\/chemistry-europe.onlinelibrary.wiley.com\/doi\/pdf\/10.1002\/cphc.202500807","content-type":"unspecified","content-version":"vor","intended-application":"similarity-checking"}],"deposited":{"date-parts":[[2026,4,27]],"date-time":"2026-04-27T06:44:13Z","timestamp":1777272253000},"score":1,"resource":{"primary":{"URL":"https:\/\/chemistry-europe.onlinelibrary.wiley.com\/doi\/10.1002\/cphc.202500807"}},"subtitle":[],"short-title":[],"issued":{"date-parts":[[2026,4,9]]},"references-count":80,"journal-issue":{"issue":"7","published-print":{"date-parts":[[2026,4,14]]}},"alternative-id":["10.1002\/cphc.202500807"],"URL":"https:\/\/doi.org\/10.1002\/cphc.202500807","archive":["Portico"],"relation":{},"ISSN":["1439-4235","1439-7641"],"issn-type":[{"value":"1439-4235","type":"print"},{"value":"1439-7641","type":"electronic"}],"subject":[],"published":{"date-parts":[[2026,4,9]]},"assertion":[{"value":"2025-11-02","order":0,"name":"received","label":"Received","group":{"name":"publication_history","label":"Publication History"}},{"value":"2026-01-31","order":2,"name":"accepted","label":"Accepted","group":{"name":"publication_history","label":"Publication History"}},{"value":"2026-04-09","order":3,"name":"published","label":"Published","group":{"name":"publication_history","label":"Publication History"}}],"article-number":"e202500807"}}