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Integrating these principles with photocatalysis is reshaping organic synthesis by introducing adaptive control over reactivity under visible light. Through H\uf8ffbonding (hydrogen bonding), \u03c0\n                    <jats:italic>\u2013<\/jats:italic>\n                    \u03c0 stacking, host\u2010guest encapsulation, charge\u2010transfer complexation, hydrophobic effects, and\n                    <jats:italic>\u03c3<\/jats:italic>\n                    \u2010hole interactions (cation\u2010\u03c0, anion\u2010\u03c0, and halogen bonding), supramolecular photocatalysts dynamically organize substrates and modulate excited\u2010state properties, thereby influencing reaction pathways and selectivity. Such assemblies can respond to changes in substrate identity, aggregation state, or irradiation conditions, enabling tunable and metal\u2010free photochemical transformations. Inspired by biological photosystems, spatial confinement and electronic communication within supramolecular architectures further unlock unconventional reactivity beyond classical photocatalysis. 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