{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,10,20]],"date-time":"2026-10-20T11:11:27Z","timestamp":1792494687486,"version":"4.5.0"},"reference-count":26,"publisher":"Wiley","issue":"9","license":[{"start":{"date-parts":[[2011,7,5]],"date-time":"2011-07-05T00:00:00Z","timestamp":1309824000000},"content-version":"vor","delay-in-days":0,"URL":"http:\/\/onlinelibrary.wiley.com\/termsAndConditions#vor"}],"content-domain":{"domain":["chemistry-europe.onlinelibrary.wiley.com"],"crossmark-restriction":true},"short-container-title":["ChemSusChem"],"published-print":{"date-parts":[[2011,9,19]]},"abstract":"Abstract<\/jats:title>\n \n A new approach to capture and store CO\n 2<\/jats:sub>\n by mineral carbonation using recyclable ammonium salts was studied. This process integrates CO\n 2<\/jats:sub>\n capture with mineral carbonation by employing NH\n 3<\/jats:sub>\n , NH\n 4<\/jats:sub>\n HSO\n 4<\/jats:sub>\n , and NH\n 4<\/jats:sub>\n HCO\n 3<\/jats:sub>\n in the capture, mineral dissolution, and carbonation steps, respectively. NH\n 4<\/jats:sub>\n HSO\n 4<\/jats:sub>\n and NH\n 3<\/jats:sub>\n can then be regenerated by thermal decomposition of (NH\n 4<\/jats:sub>\n )\n 2<\/jats:sub>\n SO\n 4<\/jats:sub>\n . The use of NH\n 4<\/jats:sub>\n HCO\n 3<\/jats:sub>\n as the source of CO\n 2<\/jats:sub>\n can avoid desorption and compression of CO\n 2<\/jats:sub>\n . The mass ratio of Mg\/NH\n 4<\/jats:sub>\n HCO\n 3<\/jats:sub>\n \/NH\n 3<\/jats:sub>\n is the key factor controlling carbonation and the optimum ratio of 1:4:2 gives a conversion of Mg ions to hydromagnesite of 95.5\u2009%. Thermogravimetric analysis studies indicated that the regeneration efficiency of NH\n 4<\/jats:sub>\n HSO\n 4<\/jats:sub>\n and NH\n 3<\/jats:sub>\n in this process is 95\u2009%. The mass balance of the process shows that about 2.63\u2005tonnes of serpentine, 0.12\u2005tonnes of NH\n 4<\/jats:sub>\n HSO\n 4<\/jats:sub>\n , 7.48\u2005tonnes of NH\n 4<\/jats:sub>\n HCO\n 3<\/jats:sub>\n , and 0.04\u2005tonnes of NH\n 3<\/jats:sub>\n are required to sequester 1\u2005tonne of CO\n 2<\/jats:sub>\n as hydromagnesite.\n <\/jats:p>","DOI":"10.1002\/cssc.201000441","type":"journal-article","created":{"date-parts":[[2011,7,5]],"date-time":"2011-07-05T12:01:28Z","timestamp":1309867288000},"page":"1291-1300","update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":124,"title":["Integration of CO\n 2<\/sub>\n Capture and Mineral Carbonation by Using Recyclable Ammonium Salts"],"prefix":"10.1002","volume":"4","author":[{"given":"Xiaolong","family":"Wang","sequence":"first","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"M. 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