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A plausible formation mechanism for the unique structures based on a seed\u2010growth process and an etching effect due to oleylamine is proposed. The formed metal\u2013semiconductor Mott\u2013Schottky heterojunction promotes electron transfer from semiconducting Ag<jats:sub>8<\/jats:sub>SnS<jats:sub>6<\/jats:sub> to metallic Ag, which catalyzes the reduction of I<jats:sub>3<\/jats:sub><jats:sup>\u2212<\/jats:sup> to I<jats:sup>\u2212<\/jats:sup>. When used as counter electrode in dye\u2010sensitized solar cells, the heterodimers show comparable performance to platinum.<\/jats:p>","DOI":"10.1002\/cssc.201403343","type":"journal-article","created":{"date-parts":[[2015,1,23]],"date-time":"2015-01-23T17:36:49Z","timestamp":1422034609000},"page":"817-820","update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":69,"title":["The Role of Mott\u2013Schottky Heterojunctions in Ag\u2013Ag<sub>8<\/sub>SnS<sub>6<\/sub> as Counter Electrodes in Dye\u2010Sensitized Solar 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