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However, the electrochemical performance of bulk\u2010type ASLBs is critically limited by the low ionic conductivity of solid electrolytes (SEs) and poor ionic contact between the active materials and SEs. Herein, highly conductive (0.14\u2005mS\u2009cm<jats:sup>\u22121<\/jats:sup>) and dry\u2010air\u2010stable SEs (Li<jats:sub>4<\/jats:sub>SnS<jats:sub>4<\/jats:sub>) are reported, which are prepared using a scalable aqueous\u2010solution process. An active material (LiCoO<jats:sub>2<\/jats:sub>) coated by solidified Li<jats:sub>4<\/jats:sub>SnS<jats:sub>4<\/jats:sub> from aqueous solutions results in a significant improvement in the electrochemical performance of ASLBs. Side\u2010effects of the exposure of LiCoO<jats:sub>2<\/jats:sub> to aqueous solutions are minimized by using predissolved Li<jats:sub>4<\/jats:sub>SnS<jats:sub>4<\/jats:sub> solution.<\/jats:p>","DOI":"10.1002\/cssc.201700409","type":"journal-article","created":{"date-parts":[[2017,5,8]],"date-time":"2017-05-08T04:25:45Z","timestamp":1494217545000},"page":"2605-2611","update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":110,"title":["Coatable Li<sub>4<\/sub>SnS<sub>4<\/sub> Solid Electrolytes Prepared from Aqueous Solutions for All\u2010Solid\u2010State Lithium\u2010Ion Batteries"],"prefix":"10.1002","volume":"10","author":[{"given":"Young Eun","family":"Choi","sequence":"first","affiliation":[{"name":"School of Energy and Chemical Engineering Department of Energy Engineering Ulsan National Institute of Science and Technology (UNIST)  Ulsan 44919 South Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Kern Ho","family":"Park","sequence":"additional","affiliation":[{"name":"School of Energy and Chemical Engineering Department of Energy Engineering Ulsan National Institute of Science and Technology (UNIST)  Ulsan 44919 South Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Dong Hyeon","family":"Kim","sequence":"additional","affiliation":[{"name":"School of Energy and Chemical Engineering Department of Energy Engineering Ulsan National Institute of Science and Technology (UNIST)  Ulsan 44919 South Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Dae Yang","family":"Oh","sequence":"additional","affiliation":[{"name":"School of Energy and Chemical Engineering Department of Energy Engineering Ulsan National Institute of Science and Technology (UNIST)  Ulsan 44919 South Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Hi Ram","family":"Kwak","sequence":"additional","affiliation":[{"name":"School of Energy and Chemical Engineering Department of Energy Engineering Ulsan National Institute of Science and Technology (UNIST)  Ulsan 44919 South Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Young\u2010Gi","family":"Lee","sequence":"additional","affiliation":[{"name":"Power Control Device Research Team Electronics and Telecommunications Research Institute (ETRI)  218 Gajeongno, Yuseong-gu Daejeon 305-700 South Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-0357-9508","authenticated-orcid":false,"given":"Yoon Seok","family":"Jung","sequence":"additional","affiliation":[{"name":"School of Energy and Chemical Engineering Department of Energy Engineering Ulsan National Institute of Science and Technology (UNIST)  Ulsan 44919 South Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2017,5,31]]},"reference":[{"key":"e_1_2_7_1_1","unstructured":"\u00a0"},{"key":"e_1_2_7_2_2","doi-asserted-by":"publisher","DOI":"10.1021\/cm901452z"},{"key":"e_1_2_7_3_2","doi-asserted-by":"publisher","DOI":"10.1038\/natrevmats.2016.103"},{"key":"e_1_2_7_4_1","unstructured":"\u00a0"},{"key":"e_1_2_7_5_2","doi-asserted-by":"publisher","DOI":"10.1038\/nmat3066"},{"key":"e_1_2_7_6_2","doi-asserted-by":"publisher","DOI":"10.1002\/ijch.201400112"},{"key":"e_1_2_7_7_2","doi-asserted-by":"publisher","DOI":"10.1038\/nenergy.2016.141"},{"key":"e_1_2_7_8_2","doi-asserted-by":"publisher","DOI":"10.1002\/adma.201505008"},{"key":"e_1_2_7_9_2","doi-asserted-by":"publisher","DOI":"10.1038\/nenergy.2016.30"},{"key":"e_1_2_7_10_2","doi-asserted-by":"publisher","DOI":"10.1038\/nmat4369"},{"key":"e_1_2_7_11_2","doi-asserted-by":"publisher","DOI":"10.1149\/2.002308jes"},{"key":"e_1_2_7_12_2","doi-asserted-by":"publisher","DOI":"10.1021\/acs.nanolett.7b00330"},{"key":"e_1_2_7_13_1","unstructured":"\u00a0"},{"key":"e_1_2_7_14_2","doi-asserted-by":"publisher","DOI":"10.1039\/C3EE41655K"},{"key":"e_1_2_7_15_2","doi-asserted-by":"publisher","DOI":"10.1149\/2.0441504jes"},{"key":"e_1_2_7_16_1","doi-asserted-by":"publisher","DOI":"10.1021\/cr030203g"},{"key":"e_1_2_7_17_1","doi-asserted-by":"publisher","DOI":"10.1021\/cm901819c"},{"key":"e_1_2_7_18_1","doi-asserted-by":"publisher","DOI":"10.1021\/acs.chemmater.6b00610"},{"key":"e_1_2_7_19_1","doi-asserted-by":"publisher","DOI":"10.1021\/cm5016959"},{"key":"e_1_2_7_20_1","first-page":"7","volume":"5","author":"Oh D. 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