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A simple, mild, and versatile method has been developed that exploits atmospheric SO<jats:sub>2<\/jats:sub> in the synthesis of porous polymers. Inspired by the chemistry of sulfonamides, contorted or bulky monomers with multiple amine groups were cross\u2010linked by SO<jats:sub>2<\/jats:sub> molecules in the presence of Et<jats:sub>3<\/jats:sub>N and I<jats:sub>2<\/jats:sub>. The sulfonamide polymers have specific surface areas up to 211\u2005m<jats:sup>2<\/jats:sup>\u2009g<jats:sup>\u22121<\/jats:sup>. In contrast to most porous polymers, the porous sulfonamide polymers (PSPs) are soluble in organic solvents, thus offering a chance to study their structures and molecular weights by liquid\u2010state NMR spectroscopy and gel\u2010permeation chromatography, respectively. Moreover, these PSPs can be easily processed into organic membranes. The current concept should encourage more studies to design porous polymers with SO<jats:sub>2<\/jats:sub> or CO<jats:sub>2<\/jats:sub> gases as linkages.<\/jats:p>","DOI":"10.1002\/cssc.201800572","type":"journal-article","created":{"date-parts":[[2018,4,23]],"date-time":"2018-04-23T16:04:51Z","timestamp":1524499491000},"page":"1751-1755","update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":15,"title":["Synthesis of Porous Sulfonamide Polymers by Capturing Atmospheric Sulfur Dioxide"],"prefix":"10.1002","volume":"11","author":[{"given":"Pengfei","family":"Zhang","sequence":"first","affiliation":[{"name":"School of Chemistry and Chemical Engineering Shanghai Jiao Tong University  Shanghai 200240 PR China"},{"name":"Chemical Sciences Division Oak Ridge National Laboratory  Oak Ridge Tennessee 37831 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