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However, the inferior electrical conductivity and unsatisfactory long\u2010term cycling performance seriously impede their large\u2010scale application in LIBs. Herein, a novel salen\u2010based porous framework polymer (SPP) with a large conjugated skeleton was constructed and utilized as anode for LIBs. Owing to its unique architecture with a large conjugated skeleton facilitating the electron transport, rich pores accelerating the organic electrolyte infiltration, and stable skeleton structure improving the long\u2010term cycling performance, SPP delivered a high specific capacity of 337\u2005mA\u2009h\u2009g<jats:sup>\u22121<\/jats:sup> at 0.1\u2005C (1\u2005C=250\u2005mA\u2009g<jats:sup>\u22121<\/jats:sup>) after 100 cycles, and robust rate capacity of 95.5\u2005mA\u2009h\u2009g<jats:sup>\u22121<\/jats:sup> at 32\u2005C. Importantly, an impressive long\u2010term cycling performance with a storage capacity of 155.7\u2005mA\u2009h\u2009g<jats:sup>\u22121<\/jats:sup> at 8\u2005C after 4000 cycles was obtained, showing a durable cyclic stability of SPP. Furthermore, the lithium storage mechanism of SPP was evaluated by ex\u2010situ X\u2010ray photoelectron spectroscopy, manifesting that the multiple active sites of C=N, \u2212OH, and benzene ring were responsible for the superior lithium storage performance. The novel SPP presented in this work should be a promising organic electrode for energy storage applications.<\/jats:p>","DOI":"10.1002\/cssc.202101623","type":"journal-article","created":{"date-parts":[[2021,8,28]],"date-time":"2021-08-28T02:54:56Z","timestamp":1630119296000},"page":"4601-4608","update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":11,"title":["A Novel Salen\u2010based Porous Framework Polymer as Durable Anode for Lithium\u2010Ion Storage"],"prefix":"10.1002","volume":"14","author":[{"given":"Xinlu","family":"Zhang","sequence":"first","affiliation":[{"name":"Shanghai Key Laboratory of Magnetic Resonance School of Physics and Electronic Science East China Normal University  No. 500 Dongchuan Road Shanghai 200241 P. R. 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