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To establish the electronic properties of pendant polymers according to structural differences, the polymers were utilized as additional hole transport layers in planar\u2010type perovskite solar cells and organic photovoltaic cells. When P4 with thiophene\u2010pyrene pendant was used as hole transport layer, all device parameters, except open\u2010circuit voltage, were significantly improved in comparison with P0 and P1 (conjugated with <jats:italic>t<\/jats:italic>\u2010butyl pyrene derivatives). Since P4 had more electrically conductive thiophene units than benzene units with fewer alkyl groups, the supramolecular assembly of P4 was found to be more favorable in electronic devices. Furthermore, devices with P4 demonstrated lower dark current than others, which could potentially be useful for charge carrier transport and sensitive photo detecting devices.<\/jats:p>","DOI":"10.1002\/cssc.202101785","type":"journal-article","created":{"date-parts":[[2021,8,30]],"date-time":"2021-08-30T08:02:05Z","timestamp":1630310525000},"page":"5167-5178","update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":10,"title":["Versatile Pendant Polymer for Selective Charge Carrier Transport via Controlling the Supramolecular Self\u2010Assembly"],"prefix":"10.1002","volume":"14","author":[{"given":"Jihyun","family":"Lim","sequence":"first","affiliation":[{"name":"School of Integrative Engineering Chung-Ang University  84 Heukseok-ro, Dongjack-gu Seoul 06974 Republic of Korea"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Min\u2010Sung","family":"Kim","sequence":"additional","affiliation":[{"name":"Department of Chemistry Hankuk University of Foreign Studies  Yongin 17035 Gyeonggi-do Republic of Korea"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Woongsik","family":"Jang","sequence":"additional","affiliation":[{"name":"School of Integrative Engineering Chung-Ang University  84 Heukseok-ro, Dongjack-gu Seoul 06974 Republic of Korea"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Jin Kuen","family":"Park","sequence":"additional","affiliation":[{"name":"Department of Chemistry Hankuk University of Foreign Studies  Yongin 17035 Gyeonggi-do Republic of Korea"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Dong Hwan","family":"Wang","sequence":"additional","affiliation":[{"name":"School of Integrative Engineering Chung-Ang University  84 Heukseok-ro, Dongjack-gu Seoul 06974 Republic of Korea"}],"role":[{"role":"author","vocabulary":"crossref"}]}],"member":"311","published-online":{"date-parts":[[2021,9,28]]},"reference":[{"key":"e_1_2_7_1_1","doi-asserted-by":"publisher","DOI":"10.1002\/anie.201806291"},{"key":"e_1_2_7_2_1","doi-asserted-by":"publisher","DOI":"10.1002\/anie.201606574"},{"key":"e_1_2_7_3_1","doi-asserted-by":"publisher","DOI":"10.1021\/acsami.7b12135"},{"key":"e_1_2_7_4_1","doi-asserted-by":"publisher","DOI":"10.1021\/acsami.5b09012"},{"key":"e_1_2_7_5_1","doi-asserted-by":"publisher","DOI":"10.1039\/C7NR08797G"},{"key":"e_1_2_7_6_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.dyepig.2020.108332"},{"key":"e_1_2_7_7_1","doi-asserted-by":"publisher","DOI":"10.1021\/acsapm.0c01325"},{"key":"e_1_2_7_8_1","doi-asserted-by":"publisher","DOI":"10.1038\/pj.2016.109"},{"key":"e_1_2_7_9_1","doi-asserted-by":"publisher","DOI":"10.1021\/acsami.0c13833"},{"key":"e_1_2_7_10_1","doi-asserted-by":"publisher","DOI":"10.1002\/adfm.201904205"},{"key":"e_1_2_7_11_1","doi-asserted-by":"publisher","DOI":"10.1002\/anie.201300371"},{"key":"e_1_2_7_12_1","doi-asserted-by":"publisher","DOI":"10.1039\/D0TA06206E"},{"key":"e_1_2_7_13_1","doi-asserted-by":"publisher","DOI":"10.1016\/S0022-2860(01)00892-4"},{"key":"e_1_2_7_14_1","doi-asserted-by":"publisher","DOI":"10.1002\/anie.201502748"},{"key":"e_1_2_7_15_1","doi-asserted-by":"publisher","DOI":"10.1002\/anie.201308396"},{"key":"e_1_2_7_16_1","doi-asserted-by":"publisher","DOI":"10.1039\/C7PY01023K"},{"key":"e_1_2_7_17_1","doi-asserted-by":"publisher","DOI":"10.1002\/pola.23092"},{"key":"e_1_2_7_18_1","first-page":"1311","volume":"7","author":"Sharma S.","year":"2017","journal-title":"J. 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