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In this study, resorcinol\u2212formaldehyde (RF), which has a relatively low bandgap and high conductivity, is introduced for photothermal catalytic generation of H<jats:sub>2<\/jats:sub>O<jats:sub>2<\/jats:sub> under ambient conditions. Owing to the promoted surface charge transfer rate under high temperature, the photosynthetic yield reaches roughly 2000\u2005\u03bc<jats:sc>m<\/jats:sc> within 40\u2005min under 400\u2005mW\u2009cm<jats:sup>\u22122<\/jats:sup> irradiation with a solar\u2010to\u2010chemical conversion (SCC) efficiency of up to 0.19\u2009% at 338\u2005K under ambient conditions, exceeding the rate of photocatalysis with a cooling system by a factor of about 2.5. Notably, the H<jats:sub>2<\/jats:sub>O<jats:sub>2<\/jats:sub> produced by RF during photothermal process was formed via a two\u2010channel pathway, leading to the overall promotion of H<jats:sub>2<\/jats:sub>O<jats:sub>2<\/jats:sub> formation. The resultant H<jats:sub>2<\/jats:sub>O<jats:sub>2<\/jats:sub> can be applied in\u2005situ for pollutant removal. This work offers a sustainable and economical route for the efficient formation of H<jats:sub>2<\/jats:sub>O<jats:sub>2<\/jats:sub>.<\/jats:p>","DOI":"10.1002\/cssc.202300015","type":"journal-article","created":{"date-parts":[[2023,3,11]],"date-time":"2023-03-11T04:54:03Z","timestamp":1678510443000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":22,"title":["Solar\u2010to\u2010H<sub>2<\/sub>O<sub>2<\/sub> Energy Conversion by the Photothermal Effect of a Polymeric Photocatalyst via a Two\u2010Channel Pathway"],"prefix":"10.1002","volume":"16","author":[{"given":"Wei","family":"Liu","sequence":"first","affiliation":[{"name":"College of Materials and Chemical Engineering Key Laboratory of Inorganic Nonmetallic Crystalline and Energy Conversion Materials China Three Gorges University  Yichang 443002 P. R. 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