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Macrocycles, including cucurbiturils, calixarene, and cyclodextrins, are cage\u2010like organic compounds (with a nanocavity that contains O and N heteroatoms) with unique potential in supercapacitors. Here, we review the applications of macrocycles in supercapacitor systems, and we illustrate the merits of organic macrocycles in electrodes and electrolytes for improving the electrochemical double\u2010layer capacitors and pseudocapacitance via supramolecular strategies. Then, the observed relationships between electrochemical performance and macrocyclic structures are introduced. This comprehensive review describes recent progress on macrocycle\u2010block supercapacitors for researchers.<\/jats:p>","DOI":"10.1002\/cssc.202300027","type":"journal-article","created":{"date-parts":[[2023,3,22]],"date-time":"2023-03-22T06:43:49Z","timestamp":1679467429000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":6,"title":["Recent Breakthroughs in Supercapacitors Boosted by Macrocycles"],"prefix":"10.1002","volume":"16","author":[{"given":"Xian\u2010Yi","family":"Jin","sequence":"first","affiliation":[{"name":"Collaborative Innovation Center of Guizhou Province for Efficient Utilization of Phosphorus and Fluorine Resources Guizhou University  Guiyang 550025 Guizhou P. R. 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