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Equimolar amounts of chemisorbed CO<jats:sub>2<\/jats:sub> in these solutions are obtained at 10\u2005bar and 40\u2009\u00b0C. Chemisorption takes place through the formation of bicarbonate in the aqueous solution using imidazolium\u2010containing phenolate. CO<jats:sub>2<\/jats:sub> is liberated by simple pressure relief and heating, regenerating the base. The enthalpy of absorption was estimated to be \u221238\u2005kJ\/mol, which is about 30\u2009% lower than the enthalpy of industrially employed aqueous solutions of MDEA (estimated at \u221253\u2005kJ\/mol using the same experimental apparatus). The physisorption of CO<jats:sub>2<\/jats:sub> becomes relevant at higher pressures (&gt;10\u2005bar) in these aqueous solutions. Combined physio\u2010 and chemisorption of up to 1.3\u2005mol\/mol at 40\u2005bar and 40\u2009\u00b0C can be attained with these aqueous zwitterionic solutions that are thermally stable and can be recycled at least 20 times.<\/jats:p>","DOI":"10.1002\/cssc.202300971","type":"journal-article","created":{"date-parts":[[2023,9,8]],"date-time":"2023-09-08T05:10:44Z","timestamp":1694149844000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":15,"title":["Zwitterionic \u201cSolutions\u201d for Reversible CO<sub>2<\/sub> Capture"],"prefix":"10.1002","volume":"16","author":[{"ORCID":"https:\/\/orcid.org\/0000-0003-4406-9088","authenticated-orcid":false,"given":"Guilherme L. P.","family":"Aydos","sequence":"first","affiliation":[{"name":"Institute of Chemistry Universidade Federal do Rio Grande do Sul\u2013UFRGS  Av. 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