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High Ni cathode, LiNi<jats:sub>x<\/jats:sub>Co<jats:sub>y<\/jats:sub>Mn<jats:sub>z<\/jats:sub>O<jats:sub>2<\/jats:sub> (NCM, x\u22650.8, x+y+z=1), have garnered significant attention owing to their high energy density. However, the limited Li\u2010ion transfer rate and transition metal cross\u2010talk to anode pose obstacles to further improvement of electrochemical performance. To tackle these challenges, metal\u2010organic frameworks (MOFs) with chelating agents are employed as additive materials for electrode. MOFs with chelating agents offer three key attributes: (1) Effective mitigation of transition metal cross\u2010talk to the anode, (2) Partial desolvation of Li<jats:sup>+<\/jats:sup> ions through MOF pores, and (3) Immobilization of anions via metal sites in the MOF. Leveraging these advantages, the chelating MOF\u2010modified NCM cathode demonstrates reduced charge transfer resistance, both in their pristine and cycled states. In addition, they exhibit significantly improved the Li\u2010ion diffusion coefficients after 100 cycles. These findings underscore the potential of MOFs with chelating agents as promising additive materials for enhancing the performance of LIBs.<\/jats:p>","DOI":"10.1002\/cssc.202400823","type":"journal-article","created":{"date-parts":[[2024,8,22]],"date-time":"2024-08-22T17:36:43Z","timestamp":1724348203000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":6,"title":["Chelated Metal\u2010Organic Frameworks for Improved the Performance of High\u2010Nickel Cathodes in Lithium\u2010Ion Batteries"],"prefix":"10.1002","volume":"18","author":[{"given":"Heeju","family":"Ahn","sequence":"first","affiliation":[{"name":"Department of Chemical Engineering and Materials Science, and Graduate Program in System Health and Engineering Ewha Womans University  Seoul 03760 Republic of Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yeonju","family":"Park","sequence":"additional","affiliation":[{"name":"Department of Chemical Engineering and Materials Science, and Graduate Program in System Health and Engineering Ewha Womans University  Seoul 03760 Republic of Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-0505-7228","authenticated-orcid":false,"given":"Kwan Woo","family":"Nam","sequence":"additional","affiliation":[{"name":"Department of Chemical Engineering and Materials Science, and Graduate Program in System Health and Engineering Ewha Womans University  Seoul 03760 Republic of Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2024,10,23]]},"reference":[{"key":"e_1_2_9_1_1","doi-asserted-by":"publisher","DOI":"10.1002\/adma.201800561"},{"key":"e_1_2_9_2_1","doi-asserted-by":"publisher","DOI":"10.1039\/c1ee01598b"},{"key":"e_1_2_9_3_1","doi-asserted-by":"publisher","DOI":"10.1002\/ese3.95"},{"key":"e_1_2_9_4_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.mattod.2014.10.040"},{"key":"e_1_2_9_5_1","doi-asserted-by":"publisher","DOI":"10.1021\/acs.chemrev.1c00565"},{"key":"e_1_2_9_6_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.rser.2018.03.002"},{"key":"e_1_2_9_7_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.jechem.2021.03.035"},{"key":"e_1_2_9_8_1","doi-asserted-by":"publisher","DOI":"10.1039\/D0TA11775G"},{"key":"e_1_2_9_9_1","doi-asserted-by":"publisher","DOI":"10.1002\/advs.202200622"},{"key":"e_1_2_9_10_1","doi-asserted-by":"publisher","DOI":"10.1039\/D3EE00441D"},{"key":"e_1_2_9_11_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.nanoen.2017.11.010"},{"key":"e_1_2_9_12_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.cej.2020.126138"},{"key":"e_1_2_9_13_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.nanoen.2020.104643"},{"key":"e_1_2_9_14_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.jpowsour.2020.228745"},{"key":"e_1_2_9_15_1","doi-asserted-by":"publisher","DOI":"10.1002\/aenm.201701682"},{"key":"e_1_2_9_16_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.ssi.2020.115292"},{"key":"e_1_2_9_17_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.electacta.2016.06.110"},{"key":"e_1_2_9_18_1","doi-asserted-by":"publisher","DOI":"10.1021\/acsami.0c18590"},{"key":"e_1_2_9_19_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.cej.2019.123975"},{"key":"e_1_2_9_20_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41560-019-0387-1"},{"key":"e_1_2_9_21_1","doi-asserted-by":"publisher","DOI":"10.1021\/acsami.6b07431"},{"key":"e_1_2_9_22_1","doi-asserted-by":"publisher","DOI":"10.1021\/acsami.7b08006"},{"key":"e_1_2_9_23_1","doi-asserted-by":"publisher","DOI":"10.1021\/acsami.0c00643"},{"key":"e_1_2_9_24_1","doi-asserted-by":"publisher","DOI":"10.1002\/anie.202106259"},{"key":"e_1_2_9_25_1","doi-asserted-by":"publisher","DOI":"10.1039\/c0cs00147c"},{"key":"e_1_2_9_26_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.nanoen.2018.04.076"},{"key":"e_1_2_9_27_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41467-019-12857-4"},{"key":"e_1_2_9_28_1","doi-asserted-by":"crossref","unstructured":"Q. 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