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In the periodic table, Cu as only the candidate can convert CO\n                    <jats:sub>2<\/jats:sub>\n                    to C\n                    <jats:sub>2+<\/jats:sub>\n                    products such as C\n                    <jats:sub>2<\/jats:sub>\n                    H\n                    <jats:sub>4<\/jats:sub>\n                    and C\n                    <jats:sub>2<\/jats:sub>\n                    H\n                    <jats:sub>5<\/jats:sub>\n                    OH due to the suitable absorption energy to reaction intermediate. However, application of Cu is limited for its low activity and poor selectivity. The tandem catalytic strategy can effectively solve the problems caused by single copper catalyst. In tandem catalysis, how to promote the formation, transport, adsorption and coupling of the important intermediate CO is the key issue to improve the selectivity of C\n                    <jats:sub>2+<\/jats:sub>\n                    products. Regulating the structure of Cu\u2010based bimetallic can effectively promote these processes to Electrochemical CO\n                    <jats:sub>2<\/jats:sub>\n                    RR on account of its synergistic effect, electronic effect and interfacial interaction. In this review, we systematically summarized the relationship between structure of Cu\u2010based bimetallic catalysts with performance of electrochemical CO\n                    <jats:sub>2<\/jats:sub>\n                    RR. More importantly, we reveal that different Cu\u2010based bimetallic structures enhance the activity and selectivity of the catalysts by regulating the processes such as the transport and adsorption of the reaction intermediate CO. Then, we proposed well\u2010effective strategies to rationally design Cu\u2010based metallic catalysts. Finally, we put forward some challenges and opportunities that Cu\u2010based bimetallic catalysts would face in the development of electrochemical CO\n                    <jats:sub>2<\/jats:sub>\n                    RR technology in the future.\n                  <\/jats:p>","DOI":"10.1002\/cssc.202402184","type":"journal-article","created":{"date-parts":[[2024,12,23]],"date-time":"2024-12-23T11:34:46Z","timestamp":1734953686000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":8,"title":["Structural Regulating of Cu\u2010Based Metallic Electrocatalysts for CO\n                    <sub>2<\/sub>\n                    to C\n                    <sub>2+<\/sub>\n                    Products Conversion"],"prefix":"10.1002","volume":"18","author":[{"given":"Jiawei","family":"Dai","sequence":"first","affiliation":[{"name":"Key Laboratory of Material Chemistry for Energy Conversion and Storage (Ministry of Education) Hubei Key Laboratory of Material Chemistry and Service Failure School of Chemistry and Chemical Engineering Huazhong University of Science and Technology  Wuhan 430074 P. 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