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Here we report the upcycling of polyethylene terephthalate (PET) plastic and CO\n                    <jats:sub>2<\/jats:sub>\n                    toward valuable potassium diformate, terephthalic acid, and H\n                    <jats:sub>2<\/jats:sub>\n                    fuel via decoupled electrolysis. This product\u2010oriented process is realized by two electrolyzers: (1)\u2005a solid\u2010state\u2010electrolyte based CO\n                    <jats:sub>2<\/jats:sub>\n                    electrolyzer and (2)\u2005a solid\u2010polymer\u2010electrolyte\u2010based PET electrolyzer. Using a bismuth\u2010based catalyst, the CO\n                    <jats:sub>2<\/jats:sub>\n                    electrolyzer showed more than 140\u2005h continuous operation at current of 250\u2005mA, resulting in 850\u2005mL pure HCOOH solution with a concentration of 683\u2005mM. Furthermore, we constructed a solid\u2010polymer\u2010electrolyte electrolyzer with an electrode area of 50\u2005cm\n                    <jats:sup>2<\/jats:sup>\n                    for the electrooxidation of ethylene glycol to formate, achieving 30\u2005A of current at ~1.9\u2005V cell voltage and 80\u2009% formate Faradaic efficiency. With this electrolyzer, we demonstrated the efficient transformation of PET hydrolysate to a mixture of terephthalate and formate. Additionally, combining CO\n                    <jats:sub>2<\/jats:sub>\n                    derived HCOOH and PET electrolyte, we obtained recycled terephthalic acid and potassium diformate. This work provides an integrated strategy for the valorization of waste carbon resources with less using external resources.\n                  <\/jats:p>","DOI":"10.1002\/cssc.202402514","type":"journal-article","created":{"date-parts":[[2024,12,30]],"date-time":"2024-12-30T06:00:32Z","timestamp":1735538432000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":9,"title":["Product Oriented Upcycling of Waste Polyethylene Terephthalate Plastic and Carbon Dioxide via Decoupled Electrolysis"],"prefix":"10.1002","volume":"18","author":[{"given":"Wei","family":"Kong","sequence":"first","affiliation":[{"name":"State Key Laboratory of Chemical Resource Engineering Beijing University of Chemical Technology  Beijing 100029 P.\u2005R. China"},{"name":"Quzhou Institute for Innovation in Resource Chemical Engineering  Quzhou 324000 P.\u2005R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yue","family":"Ren","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Chemical Resource Engineering Beijing University of Chemical Technology  Beijing 100029 P.\u2005R. China"},{"name":"Quzhou Institute for Innovation in Resource Chemical Engineering  Quzhou 324000 P.\u2005R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Kang","family":"Zou","sequence":"additional","affiliation":[{"name":"SINOPEC Research Institute of Petroleum Processing  Beijing 100083 P.\u2005R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Zishan","family":"Han","sequence":"additional","affiliation":[{"name":"SINOPEC Research Institute of Petroleum Processing  Beijing 100083 P.\u2005R. 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China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Mingfei","family":"Shao","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Chemical Resource Engineering Beijing University of Chemical Technology  Beijing 100029 P.\u2005R. China"},{"name":"Quzhou Institute for Innovation in Resource Chemical Engineering  Quzhou 324000 P.\u2005R. 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