{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,10,20]],"date-time":"2026-10-20T03:03:58Z","timestamp":1792465438569,"version":"4.5.0"},"reference-count":32,"publisher":"Wiley","issue":"12","license":[{"start":{"date-parts":[[2025,4,9]],"date-time":"2025-04-09T00:00:00Z","timestamp":1744156800000},"content-version":"vor","delay-in-days":0,"URL":"http:\/\/onlinelibrary.wiley.com\/termsAndConditions#vor"}],"content-domain":{"domain":["chemistry-europe.onlinelibrary.wiley.com"],"crossmark-restriction":true},"short-container-title":["ChemSusChem"],"published-print":{"date-parts":[[2025,6,17]]},"abstract":"<jats:p>\n                    The photocatalytic activity of graphitic carbon nitride (g\u2010C\n                    <jats:sub>3<\/jats:sub>\n                    N\n                    <jats:sub>4<\/jats:sub>\n                    ) strongly depends on its electronic structure. To design the photocatalysts with efficient charge separation and transfer property, here a benzene ring\u2010doped g\u2010C\n                    <jats:sub>3<\/jats:sub>\n                    N\n                    <jats:sub>4<\/jats:sub>\n                    via one\u2010pot thermal polycondensation of dicyandiamide and 2,4\u2010diaminobenzenesulfonic acid is reported. The carbon\u2010rich benzene ring is embedded into g\u2010C\n                    <jats:sub>3<\/jats:sub>\n                    N\n                    <jats:sub>4<\/jats:sub>\n                    , which enables the asymmetric modification of the heptazine units in g\u2010C\n                    <jats:sub>3<\/jats:sub>\n                    N\n                    <jats:sub>4<\/jats:sub>\n                    and the extension of the \u03c0\u2010conjugate system without altering its long\u2010range order structure significantly. Such molecular structure optimization effectively improves the visible light harvesting and charge carriers separation ability. A high photocatalytic hydrogen evolution rate and dye degradation performance is achieved under visible light irradiation (\u03bb\u2009&gt;\u2009420\u2009nm), which is about 8.4 and 4.4\u2010fold higher than that of pristine g\u2010C\n                    <jats:sub>3<\/jats:sub>\n                    N\n                    <jats:sub>4<\/jats:sub>\n                    , respectively. The reason for enhanced photocatalytic performance is ascribed to a favorable optical property, suppressed charge carrier recombination, and efficient charge transfer processes. This work provides a green and economical method to functionalize g\u2010C\n                    <jats:sub>3<\/jats:sub>\n                    N\n                    <jats:sub>4<\/jats:sub>\n                    using low\u2010content organic carbon molecule for efficient energy conversion\u2010related applications.\n                  <\/jats:p>","DOI":"10.1002\/cssc.202500462","type":"journal-article","created":{"date-parts":[[2025,3,26]],"date-time":"2025-03-26T00:09:00Z","timestamp":1742947740000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":50,"title":["Benzene Ring Engineering of Graphitic Carbon Nitride for Enhanced Photocatalytic Dye Degradation and Hydrogen Production from Water Splitting"],"prefix":"10.1002","volume":"18","author":[{"ORCID":"https:\/\/orcid.org\/0000-0001-9769-5619","authenticated-orcid":false,"given":"Yongbo","family":"Fan","sequence":"first","affiliation":[{"name":"Department of Applied Physics The Hong Kong Polytechnic University  Hung Hom 100872 Hong Kong"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-4899-7378","authenticated-orcid":false,"given":"Lin","family":"Lei","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Solidification Processing School of Materials Science and Engineering Northwestern Polytechnical University  Xi\u2019An 710072 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jingshen","family":"Cao","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Solidification Processing School of Materials Science and Engineering Northwestern Polytechnical University  Xi\u2019An 710072 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-0164-9322","authenticated-orcid":false,"given":"Weijia","family":"Wang","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Solidification Processing School of Materials Science and Engineering Northwestern Polytechnical University  Xi\u2019An 710072 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-1405-9279","authenticated-orcid":false,"given":"Huiqing","family":"Fan","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Solidification Processing School of Materials Science and Engineering Northwestern Polytechnical University  Xi\u2019An 710072 China"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2025,4,9]]},"reference":[{"key":"e_1_2_8_2_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.snb.2024.137072"},{"key":"e_1_2_8_3_1","doi-asserted-by":"publisher","DOI":"10.1021\/acscatal.3c05826"},{"key":"e_1_2_8_4_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.seppur.2023.125225"},{"key":"e_1_2_8_5_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.cclet.2024.109580"},{"key":"e_1_2_8_6_1","doi-asserted-by":"publisher","DOI":"10.1039\/C7CY01784G"},{"key":"e_1_2_8_7_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.seppur.2024.130880"},{"key":"e_1_2_8_8_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.chemosphere.2019.01.045"},{"key":"e_1_2_8_9_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.electacta.2024.145370"},{"key":"e_1_2_8_10_1","doi-asserted-by":"publisher","DOI":"10.1002\/adma.202005256"},{"key":"e_1_2_8_11_1","doi-asserted-by":"publisher","DOI":"10.1002\/adma.202101455"},{"key":"e_1_2_8_12_1","doi-asserted-by":"publisher","DOI":"10.1002\/adfm.202416946"},{"key":"e_1_2_8_13_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.apcatb.2022.121497"},{"key":"e_1_2_8_14_1","doi-asserted-by":"publisher","DOI":"10.1021\/jacs.6b11878"},{"key":"e_1_2_8_15_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.cej.2021.130991"},{"key":"e_1_2_8_16_1","doi-asserted-by":"publisher","DOI":"10.1002\/anie.201813117"},{"key":"e_1_2_8_17_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.joule.2018.03.006"},{"key":"e_1_2_8_18_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.ces.2024.120409"},{"key":"e_1_2_8_19_1","doi-asserted-by":"publisher","DOI":"10.1039\/D4TA00434E"},{"key":"e_1_2_8_20_1","doi-asserted-by":"publisher","DOI":"10.1021\/j100258a027"},{"key":"e_1_2_8_21_1","doi-asserted-by":"publisher","DOI":"10.1039\/D1QI01607E"},{"key":"e_1_2_8_22_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.apcatb.2024.123902"},{"key":"e_1_2_8_23_1","doi-asserted-by":"publisher","DOI":"10.1002\/adma.202307490"},{"key":"e_1_2_8_24_1","doi-asserted-by":"publisher","DOI":"10.1002\/anie.202417428"},{"key":"e_1_2_8_25_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.jmst.2020.03.086"},{"key":"e_1_2_8_26_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.seppur.2022.121170"},{"key":"e_1_2_8_27_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.apcatb.2018.08.059"},{"key":"e_1_2_8_28_1","first-page":"S1342","volume":"9","author":"Fattah\u2010Alhosseini Arab","year":"2016","journal-title":"J. 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