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Among various CO\n                    <jats:sub>2<\/jats:sub>\n                    valorization routes, catalytic CO\n                    <jats:sub>2<\/jats:sub>\n                    hydrogenation to methanol (CH\n                    <jats:sub>3<\/jats:sub>\n                    OH, CHM) has attracted intensive interest, in which indium oxide (In\n                    <jats:sub>2<\/jats:sub>\n                    O\n                    <jats:sub>3<\/jats:sub>\n                    ) stands out as a highly promising candidate due to its unique properties in stabilizing key reaction intermediates for CH\n                    <jats:sub>3<\/jats:sub>\n                    OH synthesis. However, the practical implementation of pristine In\n                    <jats:sub>2<\/jats:sub>\n                    O\n                    <jats:sub>3<\/jats:sub>\n                    is severely hindered by insufficient catalytic activity. To address the bottlenecks, a variety of multidimensional modification strategies have been rationally designed and extensively explored to tune the characteristics of In\n                    <jats:sub>2<\/jats:sub>\n                    O\n                    <jats:sub>3<\/jats:sub>\n                    \u2010based catalysts, which include modulating properties of In\n                    <jats:sub>2<\/jats:sub>\n                    O\n                    <jats:sub>3<\/jats:sub>\n                    , tailoring properties of metal promoters and regulating metal\u2013In\n                    <jats:sub>2<\/jats:sub>\n                    O\n                    <jats:sub>3<\/jats:sub>\n                    interactions. In this review, we commence with a systematic discussion of the reaction mechanisms governing CHM over In\n                    <jats:sub>2<\/jats:sub>\n                    O\n                    <jats:sub>3<\/jats:sub>\n                    \u2010based catalysts, then provide an in\u2010depth summary and critical evaluation of the modification strategies for the rational design of In\n                    <jats:sub>2<\/jats:sub>\n                    O\n                    <jats:sub>3<\/jats:sub>\n                    \u2010based catalysts, and finally highlight the most challenging issues and possible solutions in this rapidly evolving field to guide the rational design of the next\u2010generation of efficient In\n                    <jats:sub>2<\/jats:sub>\n                    O\n                    <jats:sub>3<\/jats:sub>\n                    \u2010based catalytic systems for sustainable CHM and the advancement of the circular carbon economy.\n                  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