{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,8,28]],"date-time":"2026-08-28T07:19:25Z","timestamp":1787901565477,"version":"build-2784847793"},"reference-count":52,"publisher":"Wiley","issue":"16","license":[{"start":{"date-parts":[[2026,8,17]],"date-time":"2026-08-17T00:00:00Z","timestamp":1786924800000},"content-version":"vor","delay-in-days":0,"URL":"http:\/\/onlinelibrary.wiley.com\/termsAndConditions#vor"},{"start":{"date-parts":[[2026,8,17]],"date-time":"2026-08-17T00:00:00Z","timestamp":1786924800000},"content-version":"tdm","delay-in-days":0,"URL":"http:\/\/doi.wiley.com\/10.1002\/tdm_license_1.1"}],"funder":[{"DOI":"10.13039\/501100004731","name":"Natural Science Foundation of Zhejiang Province","doi-asserted-by":"publisher","award":["LY24B040001"],"award-info":[{"award-number":["LY24B040001"]}],"id":[{"id":"10.13039\/501100004731","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":["chemistry-europe.onlinelibrary.wiley.com"],"crossmark-restriction":true},"short-container-title":["ChemSusChem"],"published-print":{"date-parts":[[2026,8,27]]},"abstract":"<jats:p>\n                    Developing high\u2010performance graphene\u2010based electrode materials through rational structural design remains a critical challenge for advanced supercapacitors. In this work, a unique molecule (DAPTO) featuring four carbonyl groups and a conjugated backbone was screened and successfully introduced into reduced graphene oxide (rGO) sheets via a one\u2010step hydrothermal process. This strategy effectively suppresses the restacking of rGO while simultaneously providing abundant pseudocapacitive active sites. Structural and morphological characterizations confirm the successful grafting of DAPTO and the formation of a stable layered architecture with enlarged interlayer spacing. By optimizing the reaction mass ratio, the optimal sample, DAPTO\u2013rGO\u20131, was identified, delivering a high specific capacitance of 680\u2009F\u2009g\n                    <jats:sup>\u22121<\/jats:sup>\n                    in a three\u2010electrode system, along with excellent rate capability and low charge\u2010transfer resistance. Furthermore, a flexible symmetric supercapacitor assembled using a PVA\/H\n                    <jats:sub>2<\/jats:sub>\n                    SO\n                    <jats:sub>4<\/jats:sub>\n                    gel electrolyte exhibits a high specific capacitance of 295\u2009F\u2009g\n                    <jats:sup>\u22121<\/jats:sup>\n                    and outstanding rate performance. The device also achieves a high energy density of 26.2\u2009Wh kg\n                    <jats:sup>\u22121<\/jats:sup>\n                    at a power density of 800\u2009W kg\n                    <jats:sup>\u22121<\/jats:sup>\n                    . This work provides valuable insights into the design of advanced graphene\u2010based electrodes.\n                  <\/jats:p>","DOI":"10.1002\/cssc.70989","type":"journal-article","created":{"date-parts":[[2026,8,17]],"date-time":"2026-08-17T08:21:28Z","timestamp":1786954888000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Rational Design for Crosslinked and Pried\u2010Open Redox\u2010Active Graphene Electrode Materials and High\u2010Performance Supercapacitors"],"prefix":"10.1002","volume":"19","author":[{"ORCID":"https:\/\/orcid.org\/0009-0008-3264-1861","authenticated-orcid":false,"given":"Jialei","family":"Bao","sequence":"first","affiliation":[{"name":"School of Chemistry and Chemical Engineering Zhejiang Sci\u2010Tech University  Hangzhou China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Siying","family":"Wu","sequence":"additional","affiliation":[{"name":"School of Chemistry and 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