{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,9,26]],"date-time":"2026-09-26T10:00:23Z","timestamp":1790416823522,"version":"4.1.0"},"reference-count":58,"publisher":"Wiley","issue":"18","license":[{"start":{"date-parts":[[2026,9,24]],"date-time":"2026-09-24T00:00:00Z","timestamp":1790208000000},"content-version":"vor","delay-in-days":0,"URL":"http:\/\/onlinelibrary.wiley.com\/termsAndConditions#vor"},{"start":{"date-parts":[[2026,9,24]],"date-time":"2026-09-24T00:00:00Z","timestamp":1790208000000},"content-version":"tdm","delay-in-days":0,"URL":"http:\/\/doi.wiley.com\/10.1002\/tdm_license_1.1"}],"funder":[{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"publisher","award":["22275030"],"award-info":[{"award-number":["22275030"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":["chemistry-europe.onlinelibrary.wiley.com"],"crossmark-restriction":true},"short-container-title":["ChemSusChem"],"published-print":{"date-parts":[[2026,9,28]]},"abstract":"<jats:p>\n                    Iodine (I\n                    <jats:sub>2<\/jats:sub>\n                    ) cathodes for aqueous Zn\u2013I\n                    <jats:sub>2<\/jats:sub>\n                    batteries suffer from sluggish redox kinetics and severe polyiodide shuttling, resulting in poor utilization and cycling stability. Herein, graphitic nitrogen\u2010enriched carbonized polymer dots (CPDs) with a core\u2013shell structure are integrated with a self\u2010supporting porous carbon framework to construct a graphitic nitrogen\u2010regulated porous carbon host. The porous framework provides abundant space for iodine accommodation and accessible pathways for mass transport, while CPDs introduce graphitic\u2010N sites that strengthen iodine\u2013host interactions and facilitate interfacial electron transfer. Their cooperative action favors a dominant direct I\n                    <jats:sub>2<\/jats:sub>\n                    \/I\n                    <jats:sup>\u2212<\/jats:sup>\n                    conversion pathway with substantially suppressed accumulation of soluble polyiodide species, thereby enabling fast iodine redox kinetics and excellent cycling stability. Benefiting from these synergistic effects, the optimized PCF\u2010CPDs\/I\n                    <jats:sub>2<\/jats:sub>\n                    \u20100.2 cathode delivers a high specific capacity of 146.1\u2009mAh\u2009g\n                    <jats:sup>\u22121<\/jats:sup>\n                    at 0.3\u2009A\u2009g\n                    <jats:sup>\u22121<\/jats:sup>\n                    with 99.6% capacity retention over 500 cycles. At 1\u2009A\u2009g\n                    <jats:sup>\u22121<\/jats:sup>\n                    , it maintains 117.5\u2009mAh\u2009g\n                    <jats:sup>\u22121<\/jats:sup>\n                    with 87.1% retention after 4000 cycles. This work demonstrates that coupling porous confinement with CPDs\u2010mediated interfacial regulation provides an effective strategy for developing high\u2010performance Zn\u2013I\n                    <jats:sub>2<\/jats:sub>\n                    batteries.\n                  <\/jats:p>","DOI":"10.1002\/cssc.71090","type":"journal-article","created":{"date-parts":[[2026,9,24]],"date-time":"2026-09-24T12:47:13Z","timestamp":1790254033000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Graphitic Nitrogen\u2010Regulated Direct I\n                    <sub>2<\/sub>\n                    \/I\n                    <sup>\u2212<\/sup>\n                    Conversion to Achieve Fast Kinetics and Stability for Zn\u2013I\n                    <sub>2<\/sub>\n                    Batteries"],"prefix":"10.1002","volume":"19","author":[{"ORCID":"https:\/\/orcid.org\/0009-0000-1066-1310","authenticated-orcid":false,"given":"Yang\u2010Yu","family":"Sun","sequence":"first","affiliation":[{"name":"Key Laboratory of Sustained and Advanced Functional Materials College of Chemistry Northeast Normal University  Changchun P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Bao\u2010Hong","family":"Xu","sequence":"additional","affiliation":[{"name":"Key Laboratory of Sustained and Advanced Functional Materials College of Chemistry Northeast Normal University  Changchun P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yan\u2010Xi","family":"Chen","sequence":"additional","affiliation":[{"name":"Key Laboratory of Sustained and Advanced Functional Materials College of Chemistry Northeast Normal University  Changchun P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Ya\u2010Qi","family":"Wang","sequence":"additional","affiliation":[{"name":"Key Laboratory of Sustained and Advanced Functional Materials College of Chemistry Northeast Normal University  Changchun P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jun\u2010Jun","family":"Liu","sequence":"additional","affiliation":[{"name":"Key Laboratory of Sustained and Advanced Functional Materials College of Chemistry Northeast Normal University  Changchun P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Ming\u2010Xiao","family":"Deng","sequence":"additional","affiliation":[{"name":"Key Laboratory of Sustained and Advanced Functional Materials College of Chemistry Northeast Normal University  Changchun P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-5113-8267","authenticated-orcid":false,"given":"Hai\u2010Zhu","family":"Sun","sequence":"additional","affiliation":[{"name":"Key Laboratory of Sustained and Advanced Functional Materials College of Chemistry Northeast Normal University  Changchun P. R. 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