{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,10,5]],"date-time":"2026-10-05T03:52:33Z","timestamp":1791172353451,"version":"4.1.0"},"reference-count":55,"publisher":"Wiley","issue":"19","license":[{"start":{"date-parts":[[2026,10,4]],"date-time":"2026-10-04T00:00:00Z","timestamp":1791072000000},"content-version":"vor","delay-in-days":0,"URL":"http:\/\/creativecommons.org\/licenses\/by-nc\/4.0\/"},{"start":{"date-parts":[[2026,10,4]],"date-time":"2026-10-04T00:00:00Z","timestamp":1791072000000},"content-version":"tdm","delay-in-days":0,"URL":"http:\/\/doi.wiley.com\/10.1002\/tdm_license_1.1"}],"content-domain":{"domain":["chemistry-europe.onlinelibrary.wiley.com"],"crossmark-restriction":true},"short-container-title":["ChemSusChem"],"published-print":{"date-parts":[[2026,10,14]]},"abstract":"<jats:p>\n                    Carbon dioxide\u2010derived polyols (CO\n                    <jats:sub>2<\/jats:sub>\n                    \u2010polyols), synthesized via the copolymerization of CO\n                    <jats:sub>2<\/jats:sub>\n                    with epoxides, have emerged as a compelling sustainable alternative to petroleum\u2010based polyols for polyurethane (PU) manufacturing, offering the dual benefit of sequestering waste CO\n                    <jats:sub>2<\/jats:sub>\n                    and reducing reliance on fossil feedstocks. However, the carbonate linkages embedded within the CO\n                    <jats:sub>2<\/jats:sub>\n                    \u2010polyol backbone impart a chain rigidity that alters intermolecular interactions and physico\u2010mechanical behavior relative to conventional polyols, creating uncertainty over how CO\n                    <jats:sub>2<\/jats:sub>\n                    incorporation translates into end\u2010use performance and slowing industrial adoption despite clear environmental incentives. This review maps the diverse application frontiers of CO\n                    <jats:sub>2<\/jats:sub>\n                    \u2010polyol\u2010derived PUs. Specifically, we highlight their critical roles in adhesives, coatings, thermal stimuli\u2010 responsive shape\u2010memory materials, waterborne PUs with enhanced hydrolytic and oxidative resistance, lithium\u2010ion battery binders, and polyurethane foams. Across these systems, we describe how tuning the carbonate unit content and polyol functionality allows the rigidity, crosslink density, and thermal transitions of the resulting PUs to be precisely engineered, often matching or exceeding the performance of conventional counterparts while retaining a favorable sustainability profile. Collectively, this review provides a practical design framework to accelerate the transition of CO\n                    <jats:sub>2<\/jats:sub>\n                    \u2010polyol\u2010based PUs from laboratory\u2010scale demonstrations to industrially viable, sustainable materials.\n                  <\/jats:p>","DOI":"10.1002\/cssc.71132","type":"journal-article","created":{"date-parts":[[2026,10,5]],"date-time":"2026-10-05T03:22:26Z","timestamp":1791170546000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Emerging Applications of CO\n                    <sub>2<\/sub>\n                    \u2010Based Polyurethanes: Bridging Material Sustainability and High\u2010Performance Engineering"],"prefix":"10.1002","volume":"19","author":[{"ORCID":"https:\/\/orcid.org\/0000-0002-9518-3190","authenticated-orcid":false,"given":"Kihyuk","family":"Sung","sequence":"first","affiliation":[{"name":"Department of Energy Systems Research Ajou University  Suwon South\u00a0Korea"},{"name":"Research Institute of Basic Science Ajou University  Suwon South\u00a0Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-4471-2328","authenticated-orcid":false,"given":"Hye\u2010Young","family":"Jang","sequence":"additional","affiliation":[{"name":"Department of Energy Systems Research Ajou University  Suwon South\u00a0Korea"},{"name":"Ajou Energy Science Research Center Ajou University  Suwon South Korea"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2026,10,4]]},"reference":[{"key":"e_1_2_13_2_1","doi-asserted-by":"crossref","first-page":"2665","DOI":"10.1039\/c2gc35928f","article-title":"What\u2019s New with CO2? 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