{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,10,23]],"date-time":"2026-10-23T03:40:58Z","timestamp":1792726858713,"version":"4.5.0"},"reference-count":42,"publisher":"Wiley","issue":"20","license":[{"start":{"date-parts":[[2026,10,22]],"date-time":"2026-10-22T00:00:00Z","timestamp":1792627200000},"content-version":"vor","delay-in-days":0,"URL":"http:\/\/onlinelibrary.wiley.com\/termsAndConditions#vor"},{"start":{"date-parts":[[2026,10,22]],"date-time":"2026-10-22T00:00:00Z","timestamp":1792627200000},"content-version":"tdm","delay-in-days":0,"URL":"http:\/\/doi.wiley.com\/10.1002\/tdm_license_1.1"}],"funder":[{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"publisher","award":["52572287"],"award-info":[{"award-number":["52572287"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"publisher","award":["52172266"],"award-info":[{"award-number":["52172266"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100003819","name":"Natural Science Foundation of Hubei Province","doi-asserted-by":"publisher","award":["2024AFB750"],"award-info":[{"award-number":["2024AFB750"]}],"id":[{"id":"10.13039\/501100003819","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":["chemistry-europe.onlinelibrary.wiley.com"],"crossmark-restriction":true},"short-container-title":["ChemSusChem"],"published-print":{"date-parts":[[2026,10,28]]},"abstract":"<jats:p>\n                    Rechargeable magnesium batteries (RMBs) are promising for large\u2010scale energy storage due to their intrinsic safety and abundant resources, yet their development remains critically hindered by the scarcity of high\u2010performance cathodes. Conversion\u2010type cathodes offer high theoretical capacity via multi\u2010electron redox, but most rely solely on cationic redox, leading to sluggish kinetics, high activation barriers, and severe structural degradation from large volume changes. Here, we report a molecular anchoring strategy using an amine\u2010terminated hyperbranched polymer (AHP) as a multifunctional template. The terminal \u2010NH\n                    <jats:sub>2<\/jats:sub>\n                    groups coordinate Co\n                    <jats:sup>2+<\/jats:sup>\n                    in situ, directing the formation of ultradispersed CoS\n                    <jats:sub>2<\/jats:sub>\n                    nanoclusters, while the AHP matrix uniformly permeates CoS\n                    <jats:sub>2<\/jats:sub>\n                    to form 3D flexible network that prevents nanocluster aggregation and provides elastic buffering to accommodate volumetric strain during conversion. Consequently, the CoS\n                    <jats:sub>2<\/jats:sub>\n                    \u2010AHP cathode delivers a high reversible capacity of 167.3\u2009 mAh\u2009g\n                    <jats:sup>\u22121<\/jats:sup>\n                    at 50\u2009mA\u2009g\n                    <jats:sup>\u22121<\/jats:sup>\n                    and retains capacity retention of 91.8% after 300 cycles at 200\u2009mA g\n                    <jats:sup>\u22121<\/jats:sup>\n                    . Crucially, ex situ characterizations confirm a synergistic reversible anion\u2010cation co\u2010redox mechanism involving Co\n                    <jats:sup>3+\/2+<\/jats:sup>\n                    \u2009\u2194\u2009Co\n                    <jats:sup>0<\/jats:sup>\n                    and S\n                    <jats:sub>2<\/jats:sub>\n                    <jats:sup>2\u2212<\/jats:sup>\n                    \u2009\u2194\u2009S\n                    <jats:sup>2\u2212<\/jats:sup>\n                    conversions. This work establishes a molecular anchoring strategy for anion\u2010rich conversion materials to synergistically boost reaction kinetics and maintain structural integrity, enabling high capacity and superior cycling stability, and offering new insight for high\u2010performance multivalent\u2010ion battery cathodes.\n                  <\/jats:p>","DOI":"10.1002\/cssc.71171","type":"journal-article","created":{"date-parts":[[2026,10,23]],"date-time":"2026-10-23T03:30:38Z","timestamp":1792726238000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Hyperbranched Polymer\u2010Anchored CoS\n                    <sub>2<\/sub>\n                    Nanoclusters Enabling Stable Dual\u2010Redox Mg\u2010Storage Mechanism"],"prefix":"10.1002","volume":"19","author":[{"given":"Hou\u2010an","family":"Zhang","sequence":"first","affiliation":[{"name":"Key Laboratory of Catalysis and Energy Materials Chemistry of Ministry of Education &amp; Hubei Key Laboratory of Catalysis and Materials Science Hubei R&amp;D Center of Hyperbranched Polmers Synthesis and Applications South\u2010Central Minzu University  Wuhan China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jianni","family":"Li","sequence":"additional","affiliation":[{"name":"Key Laboratory of Catalysis and Energy Materials Chemistry of Ministry of Education &amp; Hubei Key Laboratory of Catalysis and Materials Science Hubei R&amp;D Center of Hyperbranched Polmers Synthesis and Applications South\u2010Central Minzu University  Wuhan China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yibiao","family":"Guo","sequence":"additional","affiliation":[{"name":"Key Laboratory of Catalysis and Energy Materials Chemistry of Ministry of Education &amp; Hubei Key Laboratory of Catalysis and Materials Science Hubei R&amp;D Center of Hyperbranched Polmers Synthesis and Applications South\u2010Central Minzu University  Wuhan China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-7126-7405","authenticated-orcid":false,"given":"Fei","family":"Xu","sequence":"additional","affiliation":[{"name":"Key Laboratory of Hydraulic Machinery Transients Ministry of Education School of Power and Mechanical Engineering Wuhan University  Wuhan China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-1640-0805","authenticated-orcid":false,"given":"Daohong","family":"Zhang","sequence":"additional","affiliation":[{"name":"Key Laboratory of Catalysis and Energy Materials Chemistry of Ministry of Education &amp; Hubei Key Laboratory of Catalysis and Materials Science Hubei R&amp;D Center of Hyperbranched Polmers Synthesis and Applications South\u2010Central Minzu University  Wuhan China"},{"name":"Guangdong Provincial Laboratory of Chemistry and Fine Chemical Engineering Jieyang Center  Jieyang China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Ting","family":"Li","sequence":"additional","affiliation":[{"name":"Key Laboratory of Catalysis and Energy Materials Chemistry of Ministry of Education &amp; Hubei Key Laboratory of Catalysis and Materials Science Hubei R&amp;D Center of Hyperbranched Polmers Synthesis and Applications South\u2010Central Minzu University  Wuhan China"},{"name":"Guangdong Provincial Laboratory of Chemistry and Fine Chemical Engineering Jieyang Center  Jieyang China"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2026,10,22]]},"reference":[{"key":"e_1_2_9_2_1","doi-asserted-by":"crossref","first-page":"8804","DOI":"10.1039\/C8CS00319J","article-title":"A Critical Review of Cathodes for Rechargeable Mg Batteries","volume":"47","author":"Mao M.","year":"2018","journal-title":"Chemical Society Reviews"},{"key":"e_1_2_9_3_1","doi-asserted-by":"crossref","first-page":"646","DOI":"10.1038\/s41560-020-0655-0","article-title":"Current Status and Future Directions of Multivalent Metal\u2010Ion Batteries","volume":"5","author":"Liang Y.","year":"2020","journal-title":"Nature Energy"},{"key":"e_1_2_9_4_1","doi-asserted-by":"crossref","first-page":"35","DOI":"10.1016\/j.jma.2023.08.021","article-title":"Recent Advances in Electrochemical Performance of Mg\u2010Based Electrochemical Energy Storage Materials in Supercapacitors: Enhancement and Mechanism","volume":"12","author":"Xiao Y.","year":"2024","journal-title":"Journal of Magnesium and Alloys"},{"key":"e_1_2_9_5_1","doi-asserted-by":"crossref","first-page":"2410406","DOI":"10.1002\/adfm.202410406","article-title":"Challenges and Progress in Rechargeable Magnesium\u2010Ion Batteries: Materials, Interfaces, and Devices","volume":"34","author":"Wang D.","year":"2024","journal-title":"Advanced Functional Materials"},{"key":"e_1_2_9_6_1","doi-asserted-by":"crossref","first-page":"1859","DOI":"10.1016\/j.jma.2025.03.025","article-title":"Physical and Chemical Interfacial Engineering of Mg Anodes for Rechargeable Magnesium Batteries","volume":"13","author":"Lee H.","year":"2025","journal-title":"Journal of Magnesium and Alloys"},{"key":"e_1_2_9_7_1","doi-asserted-by":"crossref","first-page":"1971","DOI":"10.1039\/D0MH00315H","article-title":"Crystal Regulation Towards Rechargeable Magnesium Battery Cathode Materials","volume":"7","author":"Tan S.","year":"2020","journal-title":"Materials Horizons"},{"key":"e_1_2_9_8_1","doi-asserted-by":"crossref","first-page":"1255","DOI":"10.1021\/acsnano.2c09302","article-title":"Toward High\u2010Performance Mg\u2010S Batteries via a Copper Phosphide Modified Separator","volume":"17","author":"Yang Y.","year":"2023","journal-title":"ACS Nano"},{"key":"e_1_2_9_9_1","doi-asserted-by":"crossref","first-page":"11683","DOI":"10.1021\/cr500049y","article-title":"Quest for Nonaqueous Multivalent Secondary Batteries: Magnesium and Beyond","volume":"114","author":"Muldoon J.","year":"2014","journal-title":"Chemical Reviews"},{"key":"e_1_2_9_10_1","doi-asserted-by":"crossref","first-page":"4061","DOI":"10.1016\/j.jma.2025.08.034","article-title":"Anodes for Magnesium Batteries: State\u2010of\u2010the\u2010Art and Prospects. A Viewpoint","volume":"13","author":"Fichtner M.","year":"2025","journal-title":"Journal of Magnesium and Alloys"},{"key":"e_1_2_9_11_1","doi-asserted-by":"crossref","first-page":"e70124","DOI":"10.1002\/eem2.70124","article-title":"Tailoring Loose Mg 2+ Solvation Structure by Steric and Competitive Solvent Coordination for Fast\u2010Charging Magnesium Batteries","volume":"9","author":"Shen Y.","year":"2026","journal-title":"Energy Environmental Material"},{"key":"e_1_2_9_12_1","doi-asserted-by":"crossref","first-page":"100129","DOI":"10.1016\/j.revmat.2025.100129","article-title":"Boron\u2010Based Electrolytes for Rechargeable Magnesium Batteries: From Design Principles to the Optimization of Mg[B(hfip)4]2 via Additives and Solvation Modulations","volume":"1","author":"Xu K.","year":"2025","journal-title":"Review of Materials Research"},{"key":"e_1_2_9_13_1","doi-asserted-by":"crossref","first-page":"227","DOI":"10.1016\/j.ensm.2022.10.034","article-title":"Recent Progress on Cathode Materials for Rechargeable Magnesium Batteries","volume":"54","author":"Kotobuki M.","year":"2023","journal-title":"Energy Storage Materials"},{"key":"e_1_2_9_14_1","doi-asserted-by":"crossref","first-page":"1903591","DOI":"10.1002\/aenm.201903591","article-title":"Recent Advances in Rechargeable Magnesium\u2010Based Batteries for High\u2010Efficiency Energy Storage","volume":"10","author":"Guo Z.","year":"2020","journal-title":"Advanced Energy Materials"},{"key":"e_1_2_9_15_1","doi-asserted-by":"crossref","first-page":"2300682","DOI":"10.1002\/aenm.202300682","article-title":"Cathode Materials and Chemistries for Magnesium Batteries: Challenges and Opportunities","volume":"13","author":"Li Z.","year":"2023","journal-title":"Advanced Energy Materials"},{"key":"e_1_2_9_16_1","doi-asserted-by":"crossref","first-page":"100226","DOI":"10.1016\/j.actphy.2025.100226","article-title":"Recent Advances in Inorganic Cathodes for Rechargeable Magnesium Metal Batteries","volume":"42","author":"Zhu C.","year":"2026","journal-title":"Acta Physico\u2010Chimica Sinica"},{"key":"e_1_2_9_17_1","doi-asserted-by":"crossref","first-page":"1800020","DOI":"10.1002\/smtd.201800020","article-title":"Rechargeable Magnesium Batteries Using Conversion\u2010Type Cathodes: A Perspective and Minireview","volume":"2","author":"Zhang Z.","year":"2018","journal-title":"Small Methods"},{"key":"e_1_2_9_18_1","doi-asserted-by":"crossref","first-page":"2007683","DOI":"10.1002\/smll.202007683","article-title":"Designing Nanostructured Metal Chalcogenides as Cathode Materials for Rechargeable Magnesium Batteries","volume":"17","author":"Regulacio M. D.","year":"2021","journal-title":"Small"},{"key":"e_1_2_9_19_1","doi-asserted-by":"crossref","first-page":"4400","DOI":"10.1039\/D3QM00366C","article-title":"Current Material Design Strategies on the Copper Chalcogenide Cathodes for Rechargeable Magnesium Batteries: A Review","volume":"7","author":"Liu X.","year":"2023","journal-title":"Materials Chemistry Frontiers"},{"key":"e_1_2_9_20_1","doi-asserted-by":"crossref","first-page":"1329","DOI":"10.1021\/accountsmr.4c00181","article-title":"The Design of Transition Metal Sulfide Cathodes for High Performance Magnesium\u2010Ion Batteries","volume":"5","author":"Wang J.","year":"2024","journal-title":"Accounts of Materials Research"},{"key":"e_1_2_9_21_1","doi-asserted-by":"crossref","first-page":"18880","DOI":"10.1039\/C9TA05233J","article-title":"Using CoS Cathode Materials With 3D Hierarchical Porosity and an Ionic Liquid (IL) as an Electrolyte Additive for High Capacity Rechargeable Magnesium Batteries","volume":"7","author":"Pan 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Batteries","volume":"36","author":"Wang J.","year":"2026","journal-title":"Advanced Functional Materials"},{"key":"e_1_2_9_28_1","doi-asserted-by":"crossref","first-page":"16043","DOI":"10.1039\/C9NR04280F","article-title":"A\u2010MoS3@CNT Nanowire Cathode for Rechargeable Mg Batteries: A Pseudocapacitive Approach for Efficient Mg\u2010Storage","volume":"11","author":"Zhang Y.","year":"2019","journal-title":"Nanoscale"},{"key":"e_1_2_9_29_1","doi-asserted-by":"crossref","first-page":"19588","DOI":"10.1021\/jacs.0c08222","article-title":"Exploring Cation\u2013Anion Redox Processes in One\u2010Dimensional Linear Chain Vanadium Tetrasulfide Rechargeable Magnesium Ion Cathodes","volume":"142","author":"Dey S.","year":"2020","journal-title":"Journal of the American Chemical Society"},{"key":"e_1_2_9_30_1","doi-asserted-by":"crossref","first-page":"2400518","DOI":"10.1002\/sstr.202400518","article-title":"Solid\u2010State Synthesis of Phase\u2010Pure Micron\u2010Sized Patr\u00f3nite Vanadium Tetrasulfide Toward Practical Magnesium Batteries","volume":"6","author":"Reupert A.","year":"2025","journal-title":"Small Structures"},{"key":"e_1_2_9_31_1","doi-asserted-by":"crossref","first-page":"28810","DOI":"10.1021\/acsnano.4c08576","article-title":"3D Tunnel Copper Tetrathiovanadate Nanocube Cathode Achieving Ultrafast Magnesium Storage Reactions Through a Charge Delocalization and Displacement Mechanism","volume":"18","author":"Tao D.","year":"2024","journal-title":"ACS Nano"},{"key":"e_1_2_9_32_1","doi-asserted-by":"crossref","first-page":"2400903","DOI":"10.1002\/smll.202400903","article-title":"Amorphous Cobalt Polyselenides With Hyperbranched Polymer Additive as High\u2010Capacity Magnesium Storage Cathode Materials Through Cationic and Anionic Co\u2010Redox Mechanism","volume":"20","author":"Li T.","year":"2024","journal-title":"Small"},{"key":"e_1_2_9_33_1","doi-asserted-by":"crossref","first-page":"2411223","DOI":"10.1002\/adfm.202411223","article-title":"Cu3VSe4 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CoS2\/CoS Heterojunction Electrocatalysts for Aqueous Polysulfide\/Iodide Redox Flow Batteries","volume":"10","author":"Ma D.","year":"2019","journal-title":"Nature Communications"},{"key":"e_1_2_9_39_1","doi-asserted-by":"crossref","first-page":"2504","DOI":"10.1039\/C6TA09983A","article-title":"An Efficient CoS2\/CoSe2 Hybrid Catalyst for Electrocatalytic Hydrogen Evolution","volume":"5","author":"Guo Y.","year":"2017","journal-title":"Journal of Materials Chemistry A"},{"key":"e_1_2_9_40_1","doi-asserted-by":"crossref","first-page":"1800935","DOI":"10.1002\/aenm.201800935","article-title":"Ultrafine Pt Nanoparticle\u2010Decorated Pyrite\u2010Type CoS2 Nanosheet Arrays Coated on Carbon Cloth as a Bifunctional Electrode for Overall Water Splitting","volume":"8","author":"Han X.","year":"2018","journal-title":"Advanced Energy Materials"},{"key":"e_1_2_9_41_1","doi-asserted-by":"crossref","first-page":"129367","DOI":"10.1016\/j.cej.2021.129367","article-title":"TCNQ\u2010Derived N\/S 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Supercaps"}],"container-title":["ChemSusChem"],"original-title":[],"language":"en","link":[{"URL":"https:\/\/chemistry-europe.onlinelibrary.wiley.com\/doi\/pdf\/10.1002\/cssc.71171","content-type":"application\/pdf","content-version":"vor","intended-application":"text-mining"},{"URL":"https:\/\/chemistry-europe.onlinelibrary.wiley.com\/doi\/full-xml\/10.1002\/cssc.71171","content-type":"application\/xml","content-version":"vor","intended-application":"text-mining"},{"URL":"https:\/\/chemistry-europe.onlinelibrary.wiley.com\/doi\/pdf\/10.1002\/cssc.71171","content-type":"unspecified","content-version":"vor","intended-application":"similarity-checking"}],"deposited":{"date-parts":[[2026,10,23]],"date-time":"2026-10-23T03:30:44Z","timestamp":1792726244000},"score":1,"resource":{"primary":{"URL":"https:\/\/chemistry-europe.onlinelibrary.wiley.com\/doi\/10.1002\/cssc.71171"}},"subtitle":[],"short-title":[],"issued":{"date-parts":[[2026,10,22]]},"references-count":42,"journal-issue":{"issue":"20","published-print":{"date-parts":[[2026,10,28]]}},"alternative-id":["10.1002\/cssc.71171"],"URL":"https:\/\/doi.org\/10.1002\/cssc.71171","archive":["Portico"],"relation":{},"ISSN":["1864-5631","1864-564X"],"issn-type":[{"value":"1864-5631","type":"print"},{"value":"1864-564X","type":"electronic"}],"subject":[],"published":{"date-parts":[[2026,10,22]]},"assertion":[{"value":"2026-07-13","order":0,"name":"received","label":"Received","group":{"name":"publication_history","label":"Publication 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