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The present study was conducted to determine the fate and bioaccumulation of methylmercury (MeHg) to lower trophic-level taxa in the river. Surface sediment directly adjacent to the source showed significantly elevated MeHg (10\u201340\u00d7 increase, mean\u2009\u00b1\u2009standard deviation [SD]: 20.1\u2009\u00b1\u200924.8 ng g\u20131 dry wt) and total mercury (THg; 10\u201330\u00d7 increase, mean\u2009\u00b1\u2009SD: 2045\u2009\u00b1\u20092669 ng g\u20131 dry wt) compared with all other reaches, with sediment THg and MeHg from downstream reaches elevated (3\u20137\u00d7 on average) relative to the reference (THg mean\u2009\u00b1\u2009SD: 33.5\u2009\u00b1\u20099.33 ng g\u20131 dry wt; MeHg mean\u2009\u00b1\u2009SD: 0.52\u2009\u00b1\u20090.21\u2009ng g\u20131 dry wt). Water column THg concentrations adjacent to the point source for both particulate (0.23\u2009ng L\u20131) and dissolved (0.76\u2009ng L\u20131) fractions were 5-fold higher than at the reference sites, and 2-fold to 5-fold higher than downstream. Methylmercury production potential of periphyton material was highest (2\u20139\u2009ng g\u20131 d\u20131 dry wt) adjacent to the Superfund site; other reaches were close to or below reporting limits (0. 1\u2009ng g\u20131 d\u20131 dry wt). Total Hg and MeHg bioaccumulation in fauna was variable across sites and taxa, with no clear spatial patterns downstream of the contamination source. Crayfish, mayflies, and shiners showed a weak positive relationship with porewater MeHg concentration. Environ Toxicol Chem 2015;34:1649\u20131658. \u00a9 2015 SETAC<\/jats:p>\n               <\/jats:sec>","DOI":"10.1002\/etc.2964","type":"journal-article","created":{"date-parts":[[2015,3,2]],"date-time":"2015-03-02T21:51:35Z","timestamp":1425333095000},"page":"1649-1658","update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":18,"title":["Influence of a chlor-alkali superfund site on mercury bioaccumulation in periphyton and low-trophic level fauna"],"prefix":"10.1093","volume":"34","author":[{"given":"Kate L.","family":"Buckman","sequence":"first","affiliation":[{"name":"Biology DepartmentDartmouth College Hanover, New Hampshire USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Mark","family":"Marvin-DiPasquale","sequence":"additional","affiliation":[{"name":"US Geological Survey Menlo Park, California USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Vivien F.","family":"Taylor","sequence":"additional","affiliation":[{"name":"Department of Earth SciencesDartmouth College Hanover, New Hampshire USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Ann","family":"Chalmers","sequence":"additional","affiliation":[{"name":"US Geological SurveyMontpelier Vermont USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Hannah J.","family":"Broadley","sequence":"additional","affiliation":[{"name":"Biology DepartmentDartmouth College Hanover, New Hampshire USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jennifer","family":"Agee","sequence":"additional","affiliation":[{"name":"US Geological Survey Menlo Park, California USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Brian P.","family":"Jackson","sequence":"additional","affiliation":[{"name":"Department of Earth SciencesDartmouth College Hanover, New Hampshire USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Celia Y.","family":"Chen","sequence":"additional","affiliation":[{"name":"Biology DepartmentDartmouth College Hanover, New Hampshire USA"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"286","published-online":{"date-parts":[[2015,3,2]]},"reference":[{"key":"2025010316030757700_etc2964-bib-0001","doi-asserted-by":"crossref","first-page":"29","DOI":"10.1641\/B570107","article-title":"Biological mercury hotspots in the northeastern United States and southeastern Canada","volume":"57","author":"Evers","year":"2007","journal-title":"BioScience"},{"key":"2025010316030757700_etc2964-bib-0002","doi-asserted-by":"crossref","first-page":"235","DOI":"10.1289\/ehp.9377","article-title":"Mercury exposure from domestic and imported estuarine and marine fish in the US seafood market","volume":"115","author":"Sunderland","year":"2007","journal-title":"Environ Health Persp"},{"key":"2025010316030757700_etc2964-bib-0003","doi-asserted-by":"crossref","first-page":"799","DOI":"10.1289\/ehp.1104494","article-title":"Evidence on the human health effects of low level methylmercury exposure","volume":"120","author":"Karagas","year":"2012","journal-title":"Environ Health Persp"},{"key":"2025010316030757700_etc2964-bib-0004","doi-asserted-by":"crossref","first-page":"3","DOI":"10.1579\/0044-7447(2007)36[3:MEAHEI]2.0.CO;2","article-title":"Methylmercury exposure and health effects in humans: A worldwide concern","volume":"36","author":"Mergler","year":"2007","journal-title":"Ambio"},{"key":"2025010316030757700_etc2964-bib-0005","doi-asserted-by":"crossref","first-page":"69","DOI":"10.1007\/s10646-007-0168-7","article-title":"Adverse effects from environmental mercury loads on breeding common loons","volume":"17","author":"Evers","year":"2008","journal-title":"Ecotoxicology"},{"key":"2025010316030757700_etc2964-bib-0006","doi-asserted-by":"crossref","first-page":"1556","DOI":"10.1002\/etc.5620220718","article-title":"Mercury effects on predator avoidance behavior of a forage fish, golden shiner (Notemigonus crysoleucas)","volume":"22","author":"Webber","year":"2009","journal-title":"Environ Toxicol Chem"},{"key":"2025010316030757700_etc2964-bib-0007","author":"Wiener","year":"1996"},{"key":"2025010316030757700_etc2964-bib-0008","author":"Ward","year":"2010"},{"key":"2025010316030757700_etc2964-bib-0009","doi-asserted-by":"crossref","first-page":"160","DOI":"10.1016\/j.envres.2012.12.011","article-title":"Contribution of contaminated sites to the global mercury budget","volume":"125","author":"Kocman","year":"2013","journal-title":"Environ Res"},{"key":"2025010316030757700_etc2964-bib-0010","doi-asserted-by":"crossref","first-page":"1","DOI":"10.1016\/j.scitotenv.2007.02.033","article-title":"Mercury contamination in the vicinity of a derelict chlor-alkali plant. 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