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Passive sampling should allow prediction of the concentration of the chemically labile fraction of MeHg in sediment porewaters based on equilibrium partitioning into the sampler, without modeling diffusion rates through the sampler material. Our goals were to identify sampler materials with the potential to mimic MeHg partitioning into animals and sediments and provide reversible sorption in a time frame appropriate for in situ samplers. Candidate materials tested included a range of polymers embedded with suitable sorbents for MeHg. The most promising were activated carbon (AC) embedded in agarose, thiol\u2013self-assembled monolayers on mesoporous supports embedded in agarose, and cysteine-functionalized polyethylene terephthalate, which yielded log sampler\u2013water partition coefficients of 2.8 to 5 for MeHgOH and MeHg complexed with dissolved organic matter (Suwannee River humic acid). Sampler equilibration time in sediments was approximately 1 to 2\u2009wk. Investigation of the MeHg accumulation mechanism by AC embedded in agarose suggested that sampling was kinetically influenced by MeHg interactions with AC particles and not limited by diffusion through the gel for this material. Also, AC exhibited relatively rapid desorption of Hg and MeHg, indicating that this sorbent is capable of reversible, equilibrium measurements. In sediment:water microcosms, porewater concentrations made with isotherm-calibrated passive samplers agreed within a factor of 2 (unamended sediment) or 4 (AC-amended sediment) with directly measured concentrations. The present study demonstrates a potential new approach to passive sampling of MeHg. Environ Toxicol Chem 2020;39:323\u2013334. \u00a9 2019 SETAC<\/jats:p>\n               <jats:p>Abstract<\/jats:p>\n               <jats:p\/>","DOI":"10.1002\/etc.4631","type":"journal-article","created":{"date-parts":[[2019,11,6]],"date-time":"2019-11-06T12:39:21Z","timestamp":1573043961000},"page":"323-334","update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":9,"title":["Development of a Novel Equilibrium Passive Sampling Device for Methylmercury in Sediment and Soil Porewaters"],"prefix":"10.1093","volume":"39","author":[{"given":"James P.","family":"Sanders","sequence":"first","affiliation":[{"name":"Department of Chemical, Biochemical, and Environmental Engineering University of Maryland Baltimore County Baltimore Maryland USA"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Alyssa","family":"McBurney","sequence":"additional","affiliation":[{"name":"Smithsonian Environmental Research Center Edgewater Maryland USA"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Cynthia C.","family":"Gilmour","sequence":"additional","affiliation":[{"name":"Smithsonian Environmental Research Center Edgewater Maryland USA"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Grace E.","family":"Schwartz","sequence":"additional","affiliation":[{"name":"Smithsonian Environmental Research Center Edgewater Maryland USA"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Spencer","family":"Washburn","sequence":"additional","affiliation":[{"name":"Smithsonian Environmental Research Center Edgewater Maryland USA"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Susan B.","family":"Kane Driscoll","sequence":"additional","affiliation":[{"name":"Exponent Maynard Massachusetts USA"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Steven S.","family":"Brown","sequence":"additional","affiliation":[{"name":"The Dow Chemical Company Midland Michigan USA"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Upal","family":"Ghosh","sequence":"additional","affiliation":[{"name":"Department of Chemical, Biochemical, and Environmental Engineering University of Maryland Baltimore County Baltimore Maryland USA"}],"role":[{"role":"author","vocabulary":"crossref"}]}],"member":"286","published-online":{"date-parts":[[2019,11,6]]},"reference":[{"key":"2025010314155685300_etc4631-bib-0001","doi-asserted-by":"crossref","first-page":"3196","DOI":"10.1021\/es103992s","article-title":"Influence of dissolved organic matter on the environmental fate of metals, nanoparticles, and colloids","volume":"45","author":"Aiken","year":"2011","journal-title":"Environ Sci Technol"},{"key":"2025010314155685300_etc4631-bib-0002","doi-asserted-by":"crossref","first-page":"2104","DOI":"10.1039\/c3em00355h","article-title":"Assessment of mercury bioavailability to benthic macroinvertebrates using diffusive gradients in thin films (DGT)","volume":"15","author":"Amirbahman","year":"2013","journal-title":"Environ Sci Process Impacts"},{"key":"2025010314155685300_etc4631-bib-0003","doi-asserted-by":"crossref","first-page":"3911","DOI":"10.1021\/es990365n","article-title":"Atomic force microscopy of humic substances: Effects of pH and ionic strength","volume":"33","author":"Balnois","year":"1999","journal-title":"Environ Sci Technol"},{"key":"2025010314155685300_etc4631-bib-0004","doi-asserted-by":"crossref","first-page":"127","DOI":"10.1021\/es001415n","article-title":"The influence of sulfide on solid phase mercury bioavailability for methylation by pure cultures of Desulfobulbus propionicus (1pr3)","volume":"35","author":"Benoit","year":"2001","journal-title":"Environ Sci Technol"},{"key":"2025010314155685300_etc4631-bib-0005","doi-asserted-by":"crossref","first-page":"277","DOI":"10.1016\/S0168-3659(01)00227-9","article-title":"Improvement in the mucoadhesive properties of alginate by the covalent attachment of cysteine","volume":"71","author":"Bernkop-Schn\u00fcrch","year":"2001","journal-title":"J Control Release"},{"key":"2025010314155685300_etc4631-bib-0006","doi-asserted-by":"crossref","first-page":"285","DOI":"10.1590\/S1984-82502013000200010","article-title":"Synthesis and characterization of a cysteine xyloglucan conjugate as mucoadhesive polymer","volume":"49","author":"Bhalekar","year":"2013","journal-title":"Braz J Pharm Sci"},{"key":"2025010314155685300_etc4631-bib-0007","doi-asserted-by":"crossref","first-page":"249","DOI":"10.1002\/ieam.1822","article-title":"Biogeochemical controls on methylmercury in soils and sediments: Implications for site management","volume":"13","author":"Bigham","year":"2016","journal-title":"Integr Environ Assess Manag"},{"key":"2025010314155685300_etc4631-bib-0008","doi-asserted-by":"crossref","first-page":"2836","DOI":"10.1021\/ja01203a066","article-title":"The exchange adsorption of ions from aqueous solutions by organic zeolites. 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