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Transverse Micro\u2010Radiography (TMR) analysis followed at treatment conclusion to determine mineral loss and lesion depth. The remineralization process illustrated a complex interplay between surface and subsurface mineral deposition, confining the thermal\u2010wave centroid toward the dominating layer. Experimental amplitudes and phases were fitted to a coupled diffuse\u2010photon\u2010density\u2010wave and thermal\u2010wave theoretical model used to quantitatively evaluate evolving changes in thermal and optical properties of de\/remineralized enamel lesions. Additional information obtained from the LUM data corroborated the remineralization kinetics affecting the PTR signals. The results pointed to enhanced effectiveness of subsurface lesion remineralization in the presence of fluoride. (\u00a9 2011 WILEY\u2010VCH Verlag GmbH &amp; Co. 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