{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,9,30]],"date-time":"2026-09-30T20:51:19Z","timestamp":1790801479919,"version":"4.1.0"},"reference-count":36,"publisher":"Wiley","issue":"9","license":[{"start":{"date-parts":[[2024,7,9]],"date-time":"2024-07-09T00:00:00Z","timestamp":1720483200000},"content-version":"vor","delay-in-days":0,"URL":"http:\/\/creativecommons.org\/licenses\/by\/4.0\/"},{"start":{"date-parts":[[2024,7,9]],"date-time":"2024-07-09T00:00:00Z","timestamp":1720483200000},"content-version":"tdm","delay-in-days":0,"URL":"http:\/\/doi.wiley.com\/10.1002\/tdm_license_1.1"}],"funder":[{"DOI":"10.13039\/501100001659","name":"Deutsche Forschungsgemeinschaft","doi-asserted-by":"publisher","award":["428490203"],"award-info":[{"award-number":["428490203"]}],"id":[{"id":"10.13039\/501100001659","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":["onlinelibrary.wiley.com"],"crossmark-restriction":true},"short-container-title":["Journal of Biophotonics"],"published-print":{"date-parts":[[2024,9]]},"abstract":"<jats:title>Abstract<\/jats:title>\n                  <jats:p>\n                    Spontaneous Raman spectroscopy is a well\u2010established diagnostic tool, allowing for the identification of all Raman active species with a single measurement. Yet, it may suffer from low\u2010signal intensity and fluorescent background. In contrast, coherent anti\u2010Stokes Raman scattering (CARS) offers laser\u2010like signals, but the traditional approach lacks the multiplex capability of spontaneous Raman spectroscopy. We present an ultrabroadband CARS setup which aims at exciting the full spectrum (300\u20133700\u2009cm\n                    <jats:sup>\u22121<\/jats:sup>\n                    ) of biological molecules. A dual\u2010output optical parametric amplifier provides a ~7\u2009fs pump\/Stokes and a\u2009~700\u2009fs probe pulse. CARS spectra of DMSO, ethanol, and methanol show great agreement with spontaneous Raman spectroscopy and superiority in fluorescent environments. The spectral resolution proves sufficient to differentiate between the complex spectra of L\u2010proline and hydroxyproline. Moreover, decay constants in the sub picosecond range are determined for individual Raman transitions, providing an additional approach for sample characterization.\n                    <jats:inline-graphic xmlns:xlink=\"http:\/\/www.w3.org\/1999\/xlink\" xlink:href=\"graphic\/jbio202300505-gra-0001.png\" xlink:title=\"image\"\/>\n                  <\/jats:p>","DOI":"10.1002\/jbio.202300505","type":"journal-article","created":{"date-parts":[[2024,7,9]],"date-time":"2024-07-09T23:36:08Z","timestamp":1720568168000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":8,"title":["Ultrabroadband two\u2010beam coherent anti\u2010Stokes Raman scattering and spontaneous Raman spectroscopy of organic fluids: A comparative study"],"prefix":"10.1002","volume":"17","author":[{"given":"Timea","family":"Koch","sequence":"first","affiliation":[{"name":"Institute of Applied Physics, Abbe Center of Photonics Friedrich\u2010Schiller\u2010Universit\u00e4t Jena  Jena Germany"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-1239-4305","authenticated-orcid":false,"given":"Roland","family":"Ackermann","sequence":"additional","affiliation":[{"name":"Institute of Applied Physics, Abbe Center of Photonics Friedrich\u2010Schiller\u2010Universit\u00e4t Jena  Jena Germany"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Axel","family":"Stoecker","sequence":"additional","affiliation":[{"name":"Faculty of Engineering and Health University of Applied Science and Arts  Goettingen Germany"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Tobias","family":"Meyer\u2010Zedler","sequence":"additional","affiliation":[{"name":"Institute of Physical Chemistry and Abbe Center of Photonics Friedrich\u2010Schiller\u2010Universit\u00e4t Jena  Jena Germany"},{"name":"Leibniz Institute of Photonic Technology  Jena Germany"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Thomas","family":"Gabler","sequence":"additional","affiliation":[{"name":"Institute of Applied Physics, Abbe Center of Photonics Friedrich\u2010Schiller\u2010Universit\u00e4t Jena  Jena Germany"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Tom","family":"Lippoldt","sequence":"additional","affiliation":[{"name":"Institute of Applied Physics, Abbe Center of Photonics Friedrich\u2010Schiller\u2010Universit\u00e4t Jena  Jena Germany"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jeannine","family":"Missbach\u2010Guentner","sequence":"additional","affiliation":[{"name":"Department of Diagnostic and Interventional Radiology University Medical Center  Goettingen Germany"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Christoph","family":"Russmann","sequence":"additional","affiliation":[{"name":"Faculty of Engineering and Health University of Applied Science and Arts  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