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The objectives of this investigation were to define the electrochemical behavior of a specific Zr\u2010based BMG alloy in a physiologically relevant environment and to compare these properties to standard, crystalline biomaterials as well as other Zr\u2010based BMG compositions. Cyclic\u2010anodic\u2010polarization studies were conducted with a Zr<jats:sub>52.5<\/jats:sub>Cu<jats:sub>17.9<\/jats:sub>Ni<jats:sub>14.6<\/jats:sub>Al<jats:sub>10.0<\/jats:sub>Ti<jats:sub>5.0<\/jats:sub>(at %) BMG in a phosphate\u2010buffered saline electrolyte with a physiologically relevant oxygen content at 37\u00b0C. The results were compared to three common, crystalline biomaterials: CoCrMo, 316L stainless steel, and Ti\u20106Al\u20104V. The BMG alloy was found to have a lower corrosion penetration rate (CPR), as compared to the 316L stainless steel, and an equivalent CPR, as compared to the CoCrMo and Ti\u20106Al\u20104V alloys. Furthermore, the BMG alloy demonstrated better localized corrosion resistance than the 316L stainless steel. However, the localized corrosion resistance of the BMG alloy was not as high as those of the CoCrMo and Ti\u20106Al\u20104V alloys in the tested environment. The excellent electrochemical properties demonstrated by the BMG alloy are combined with a low modulus and unparalleled strength. This unique combination of properties dramatically demonstrates the potential for amorphous alloys as a new generation of biomaterials. \u00a9 2005 Wiley Periodicals, Inc. 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