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In combination with already established protocols in <jats:sup>13\/14<\/jats:sup>C\u2010 or <jats:sup>11<\/jats:sup>C\u2010isotope chemistry, this manuscript should help isotope scientists to choose the best possible method for their scientific cyanation problem, but with the main focus on <jats:sup>14<\/jats:sup>C\u2010applications. 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