{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,5,9]],"date-time":"2026-05-09T17:10:40Z","timestamp":1778346640344,"version":"3.51.4"},"reference-count":60,"publisher":"Wiley","issue":"8","license":[{"start":{"date-parts":[[2026,3,10]],"date-time":"2026-03-10T00:00:00Z","timestamp":1773100800000},"content-version":"vor","delay-in-days":0,"URL":"http:\/\/onlinelibrary.wiley.com\/termsAndConditions#vor"},{"start":{"date-parts":[[2026,3,10]],"date-time":"2026-03-10T00:00:00Z","timestamp":1773100800000},"content-version":"tdm","delay-in-days":0,"URL":"http:\/\/doi.wiley.com\/10.1002\/tdm_license_1.1"}],"content-domain":{"domain":["scijournals.onlinelibrary.wiley.com"],"crossmark-restriction":true},"short-container-title":["J Sci Food Agric"],"published-print":{"date-parts":[[2026,6]]},"abstract":"<jats:title>Abstract<\/jats:title>\n                  <jats:sec>\n                    <jats:title>BACKGROUND<\/jats:title>\n                    <jats:p>Sucralose (4,1\u2032,6\u2032\u2010trichlorogalactosucrose, TGS) has been widely used as a new generation of artificial sweetener, and the loading, release and purification of TGS with edible porous materials such as cyclodextrin metal\u2013organic frameworks (CD\u2010MOF) will pave a new way for the production and application of TGS.<\/jats:p>\n                  <\/jats:sec>\n                  <jats:sec>\n                    <jats:title>RESULTS<\/jats:title>\n                    <jats:p>\n                      K\/Na\u2010\u03b2\u2010CD\u2010MOFs have been used in the loading, release and purification of TGS. TGS loading capacity of K\u2010\u03b2\u2010CD\u2010MOF is higher than that of Na\u2010\u03b2\u2010CD\u2010MOF, and the loading ratios increase with the decrease of particle size (the highest ratio is 18.00% below a size of 8.56\u2009\u03bcm). Besides, the excellent controllable TGS releasing performance can be found in nano\u2010sized K\u2010\u03b2\u2010CD\u2010MOF, during which only 41.12% TGS were released after 24\u2009h. The good loading\/releasing performance could be explained by the coordination\u2010driven ligand\u2010exchange (ethanol and TGS) in \u03b2\u2010CD\u2010MOFs, during which the weak K\uf8ffO\n                      <jats:sub>ethanol<\/jats:sub>\n                      bonds were replaced by relatively strong K\uf8ffCl\n                      <jats:sub>TGS<\/jats:sub>\n                      bonds. Finally, these \u03b2\u2010CD\u2010MOFs can adsorb DH\u20104,1\u2032\u2010DGS (3\u2032,6\u2032\u2010dehydration\u20104,1\u2032\u2010dichlorogalactosucralose, main by\u2010product in TGS production) in a TGS\/DGS mixture selectively, rending a high separation factor\n                      <jats:italic>\u03b1<\/jats:italic>\n                      of 21.39. The remarkable purifying performance stems from the smaller molecular size of DH\u20104,1\u2032\u2010DGS and less steric hindrance after dehydrating on 3\u2032,6\u2032\u2010positions.\n                    <\/jats:p>\n                  <\/jats:sec>\n                  <jats:sec>\n                    <jats:title>CONCLUSION<\/jats:title>\n                    <jats:p>\u03b2\u2010CD\u2010MOFs exhibit excellent TGS loading\/releasing performance induced by a coordination\u2010driven process, and they can purify the TGS\/DGS mixture with high efficiency. The simultaneous realization of loading\/purification of TGS on a cheap and edible material will pave a new avenue for the postprocessing of TGS. \u00a9 2026 Society of Chemical Industry.<\/jats:p>\n                  <\/jats:sec>","DOI":"10.1002\/jsfa.70572","type":"journal-article","created":{"date-parts":[[2026,3,11]],"date-time":"2026-03-11T03:25:52Z","timestamp":1773199552000},"page":"4890-4900","update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Coordination\u2010driven high sucralose loading, releasing and purifying performance of edible \u03b2\u2010cyclodextrin metal\u2013organic frameworks"],"prefix":"10.1002","volume":"106","author":[{"given":"Huimin","family":"Jie","sequence":"first","affiliation":[{"name":"Engineering Research Center of Advanced Manufacturing Technology for Fine Chemicals (Fujian Province University), College of Chemical Engineering, Fuzhou University  Fuzhou PR China"},{"name":"Fujian Huazhi Engineering Technology Co., Ltd  Fuzhou PR China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Wanfen","family":"Zeng","sequence":"additional","affiliation":[{"name":"Engineering Research Center of Advanced Manufacturing Technology for Fine Chemicals (Fujian Province University), College of Chemical Engineering, Fuzhou University  Fuzhou PR China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Zhoulin","family":"Lv","sequence":"additional","affiliation":[{"name":"College of Chemistry Fuzhou University  Fuzhou PR China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Jingjing","family":"Chen","sequence":"additional","affiliation":[{"name":"Engineering Research Center of Advanced Manufacturing Technology for Fine Chemicals (Fujian Province University), College of Chemical Engineering, Fuzhou University  Fuzhou PR China"},{"name":"Qingyuan Innovation Laboratory  Quanzhou PR China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Xiaoping","family":"Chen","sequence":"additional","affiliation":[{"name":"Engineering Research Center of Advanced Manufacturing Technology for Fine Chemicals (Fujian Province University), College of Chemical Engineering, Fuzhou University  Fuzhou PR China"},{"name":"Qingyuan Innovation Laboratory  Quanzhou PR China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Zi'ang","family":"Chen","sequence":"additional","affiliation":[{"name":"Fujian Key Laboratory of Bio\u2010based Food and Daily Chemical Additives, Techno Food Ingredients Co., Ltd  Sanming PR China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Huadong","family":"Luo","sequence":"additional","affiliation":[{"name":"Fujian Key Laboratory of Bio\u2010based Food and Daily Chemical Additives, Techno Food Ingredients Co., Ltd  Sanming PR China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Haohong","family":"Li","sequence":"additional","affiliation":[{"name":"Engineering Research Center of Advanced Manufacturing Technology for Fine Chemicals (Fujian Province University), College of Chemical Engineering, Fuzhou University  Fuzhou PR China"},{"name":"College of Chemistry Fuzhou University  Fuzhou PR China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-8346-7284","authenticated-orcid":false,"given":"Huidong","family":"Zheng","sequence":"additional","affiliation":[{"name":"Engineering Research Center of Advanced Manufacturing Technology for Fine Chemicals (Fujian Province University), College of Chemical Engineering, Fuzhou University  Fuzhou PR China"},{"name":"Qingyuan Innovation Laboratory  Quanzhou PR China"}],"role":[{"role":"author","vocabulary":"crossref"}]}],"member":"311","published-online":{"date-parts":[[2026,3,10]]},"reference":[{"key":"e_1_2_9_2_1","doi-asserted-by":"publisher","DOI":"10.1016\/S0278-6915(00)00035-1"},{"key":"e_1_2_9_3_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.comptc.2012.12.017"},{"key":"e_1_2_9_4_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.fct.2019.110898"},{"key":"e_1_2_9_5_1","doi-asserted-by":"publisher","DOI":"10.1111\/j.1365-2621.1990.tb06061.x"},{"key":"e_1_2_9_6_1","first-page":"13","article-title":"Synthesis of strong sweetener sucralose","volume":"2","author":"Luo Y","year":"2009","journal-title":"Mod Appl Sci"},{"key":"e_1_2_9_7_1","doi-asserted-by":"publisher","DOI":"10.1002\/(SICI)1097-0290(19991005)65:1<10::AID-BIT2>3.0.CO;2-L"},{"key":"e_1_2_9_8_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.foodchem.2016.02.099"},{"key":"e_1_2_9_9_1","unstructured":"MuftiKSandKhanRA Process for the preparation of 4 1\u2032 6\u2032\u2010trichloro\u20104 1\u2032 6\u2032\u2010trideoxygalactosucrose (TGS). United States Patent4380476(1983)."},{"key":"e_1_2_9_10_1","unstructured":"HoDLandWanZ Methods for extracting and purifying sucralose intermediate United States Patent 0022765(2010)."},{"key":"e_1_2_9_11_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.seppur.2022.122027"},{"key":"e_1_2_9_12_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.cej.2024.158949"},{"key":"e_1_2_9_13_1","doi-asserted-by":"publisher","DOI":"10.1007\/s11095-016-2059-1"},{"key":"e_1_2_9_14_1","doi-asserted-by":"publisher","DOI":"10.1039\/C9CS00778D"},{"key":"e_1_2_9_15_1","doi-asserted-by":"publisher","DOI":"10.1021\/acsami.9b17000"},{"key":"e_1_2_9_16_1","doi-asserted-by":"publisher","DOI":"10.1021\/acs.inorgchem.9b01740"},{"key":"e_1_2_9_17_1","doi-asserted-by":"publisher","DOI":"10.1039\/C7TB02970E"},{"key":"e_1_2_9_18_1","doi-asserted-by":"publisher","DOI":"10.1039\/b802426j"},{"key":"e_1_2_9_19_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.foodchem.2022.132605"},{"key":"e_1_2_9_20_1","doi-asserted-by":"publisher","DOI":"10.1021\/acs.accounts.0c00695"},{"key":"e_1_2_9_21_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.foodchem.2022.132467"},{"key":"e_1_2_9_22_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.crfs.2022.10.025"},{"key":"e_1_2_9_23_1","doi-asserted-by":"publisher","DOI":"10.1039\/C7RA06558B"},{"key":"e_1_2_9_24_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.tifs.2020.08.009"},{"key":"e_1_2_9_25_1","doi-asserted-by":"publisher","DOI":"10.1021\/ja208224f"},{"key":"e_1_2_9_26_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.molstruc.2015.08.020"},{"key":"e_1_2_9_27_1","doi-asserted-by":"publisher","DOI":"10.1002\/anie.201002343"},{"key":"e_1_2_9_28_1","doi-asserted-by":"publisher","DOI":"10.1002\/anie.201204919"},{"key":"e_1_2_9_29_1","doi-asserted-by":"publisher","DOI":"10.1021\/ja0627444"},{"key":"e_1_2_9_30_1","doi-asserted-by":"publisher","DOI":"10.1021\/cg101130m"},{"key":"e_1_2_9_31_1","doi-asserted-by":"publisher","DOI":"10.1021\/cr200304e"},{"key":"e_1_2_9_32_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.chroma.2025.466066"},{"key":"e_1_2_9_33_1","doi-asserted-by":"publisher","DOI":"10.1107\/S0108767307043930"},{"key":"e_1_2_9_34_1","doi-asserted-by":"publisher","DOI":"10.1107\/S0021889802022112"},{"key":"e_1_2_9_35_1","doi-asserted-by":"publisher","DOI":"10.1002\/jcc.21334"},{"key":"e_1_2_9_36_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.poly.2018.11.043"},{"key":"e_1_2_9_37_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.ccr.2021.214234"},{"key":"e_1_2_9_38_1","doi-asserted-by":"publisher","DOI":"10.1002\/chem.202402068"},{"key":"e_1_2_9_39_1","doi-asserted-by":"publisher","DOI":"10.1002\/chem.201805548"},{"key":"e_1_2_9_40_1","doi-asserted-by":"publisher","DOI":"10.1039\/D3DT00890H"},{"key":"e_1_2_9_41_1","doi-asserted-by":"publisher","DOI":"10.5650\/jos.59.601"},{"key":"e_1_2_9_42_1","doi-asserted-by":"publisher","DOI":"10.1021\/acs.langmuir.4c04860"},{"key":"e_1_2_9_43_1","doi-asserted-by":"publisher","DOI":"10.1039\/C7CC03471G"},{"key":"e_1_2_9_44_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.foodchem.2021.131760"},{"key":"e_1_2_9_45_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.cattod.2015.04.017"},{"key":"e_1_2_9_46_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.tifs.2005.11.007"},{"key":"e_1_2_9_47_1","doi-asserted-by":"publisher","DOI":"10.1021\/acsami.0c08594"},{"key":"e_1_2_9_48_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.carbpol.2025.123684"},{"key":"e_1_2_9_49_1","doi-asserted-by":"publisher","DOI":"10.2174\/0109298673328126241003092124"},{"key":"e_1_2_9_50_1","doi-asserted-by":"publisher","DOI":"10.1021\/accountsmr.3c00169"},{"key":"e_1_2_9_51_1","doi-asserted-by":"publisher","DOI":"10.1021\/ja00077a013"},{"key":"e_1_2_9_52_1","doi-asserted-by":"publisher","DOI":"10.1134\/S1063774508020053"},{"key":"e_1_2_9_53_1","doi-asserted-by":"publisher","DOI":"10.1021\/ic070328u"},{"key":"e_1_2_9_54_1","doi-asserted-by":"publisher","DOI":"10.1002\/advs.202306599"},{"key":"e_1_2_9_55_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.cej.2025.166366"},{"key":"e_1_2_9_56_1","doi-asserted-by":"publisher","DOI":"10.1039\/c3cp00054k"},{"key":"e_1_2_9_57_1","doi-asserted-by":"publisher","DOI":"10.1021\/acs.chemrev.5b00560"},{"key":"e_1_2_9_58_1","doi-asserted-by":"publisher","DOI":"10.1021\/acs.jpclett.1c03069"},{"key":"e_1_2_9_59_1","doi-asserted-by":"publisher","DOI":"10.1021\/jacs.1c03943"},{"key":"e_1_2_9_60_1","doi-asserted-by":"publisher","DOI":"10.1039\/D0TB02146F"},{"key":"e_1_2_9_61_1","doi-asserted-by":"publisher","DOI":"10.1021\/jp8111556"}],"container-title":["Journal of the Science of Food and Agriculture"],"original-title":[],"language":"en","link":[{"URL":"https:\/\/scijournals.onlinelibrary.wiley.com\/doi\/pdf\/10.1002\/jsfa.70572","content-type":"application\/pdf","content-version":"vor","intended-application":"text-mining"},{"URL":"https:\/\/scijournals.onlinelibrary.wiley.com\/doi\/full-xml\/10.1002\/jsfa.70572","content-type":"application\/xml","content-version":"vor","intended-application":"text-mining"},{"URL":"https:\/\/scijournals.onlinelibrary.wiley.com\/doi\/pdf\/10.1002\/jsfa.70572","content-type":"unspecified","content-version":"vor","intended-application":"similarity-checking"}],"deposited":{"date-parts":[[2026,5,9]],"date-time":"2026-05-09T16:29:37Z","timestamp":1778344177000},"score":1,"resource":{"primary":{"URL":"https:\/\/scijournals.onlinelibrary.wiley.com\/doi\/10.1002\/jsfa.70572"}},"subtitle":[],"short-title":[],"issued":{"date-parts":[[2026,3,10]]},"references-count":60,"journal-issue":{"issue":"8","published-print":{"date-parts":[[2026,6]]}},"alternative-id":["10.1002\/jsfa.70572"],"URL":"https:\/\/doi.org\/10.1002\/jsfa.70572","archive":["Portico"],"relation":{},"ISSN":["0022-5142","1097-0010"],"issn-type":[{"value":"0022-5142","type":"print"},{"value":"1097-0010","type":"electronic"}],"subject":[],"published":{"date-parts":[[2026,3,10]]},"assertion":[{"value":"2025-08-08","order":0,"name":"received","label":"Received","group":{"name":"publication_history","label":"Publication History"}},{"value":"2026-02-20","order":2,"name":"accepted","label":"Accepted","group":{"name":"publication_history","label":"Publication History"}},{"value":"2026-03-10","order":3,"name":"published","label":"Published","group":{"name":"publication_history","label":"Publication History"}}]}}