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Quantitative functionalization by a series of monofunctionalized ethylene glycol oligomers, from dimer to hexamer, as well as with high molecular weight polyethylene glycol is demonstrated. The length of the ethylene glycol sidechains is shown to have a direct impact on the surface wettability of the polymer, as well as its solubility in polar solvents. However, the energetics and band gap of the CPs remain essentially constant. This method therefore allows an easy way to modulate the wettability and solubility of CP materials for a diverse series of applications.<\/jats:p>","DOI":"10.1002\/mabi.202000087","type":"journal-article","created":{"date-parts":[[2020,6,15]],"date-time":"2020-06-15T08:34:54Z","timestamp":1592210094000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":24,"title":["Tunable Control of the Hydrophilicity and Wettability of Conjugated Polymers by a Postpolymerization Modification Approach"],"prefix":"10.1002","volume":"20","author":[{"given":"Shengyu","family":"Cong","sequence":"first","affiliation":[{"name":"Department of Chemistry and Centre for Processable Electronics Imperial College London  White City Campus London W12 0BZ UK"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Adam","family":"Creamer","sequence":"additional","affiliation":[{"name":"Department of Chemistry and Centre for Processable Electronics Imperial College London  White City Campus London W12 0BZ UK"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Zhuping","family":"Fei","sequence":"additional","affiliation":[{"name":"Institute of Molecular Plus Tianjin Key Laboratory of Molecular Optoelectronic Science Tianjin University  Tianjin 300072 P. 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