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The result shows that silicon\u2010carbon asymmetric side chains can modulate the aggregation degree of polymer chains with a coherence length of 134 \u00c5 and maintain the mobility at 0.90 cm<jats:sup>2<\/jats:sup> V<jats:sup>\u22121<\/jats:sup> s<jats:sup>\u22121<\/jats:sup>. P(C\u2010Si) exhibits superior tensile properties that even elongation up to 100% the value of mobility retains a majority properties. The main reason is that the lowest coherence length of P(C\u2010Si) polymer leads to an increased proportion of amorphous zones in its polymer film, which efficiently dissipates mechanical stresses. This study provides an efficient strategy for the design and synthesis of the CPs with high carrier transport properties\u2010mechanical stability.<\/jats:p>","DOI":"10.1002\/marc.202100636","type":"journal-article","created":{"date-parts":[[2021,11,30]],"date-time":"2021-11-30T23:26:58Z","timestamp":1638314818000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":14,"title":["Asymmetric Hybrid Siloxane Side Chains for Enhanced Mobility and Mechanical Properties of Diketopyrrolopyrrole\u2010Based Polymers"],"prefix":"10.1002","volume":"43","author":[{"given":"Ye","family":"Yuan","sequence":"first","affiliation":[{"name":"National Engineering Lab of Special Display Technology State Key Lab of Advanced Display Technology Academy of Opto\u2010Electronic Technology Hefei University of Technology  Hefei 230009 China"},{"name":"Anhui Province Key Laboratory of Advanced Functional Materials and Devices Hefei University of Technology  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