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With prolonged skin contact, commercial adhesives have been shown to cause allergic contact dermatitis as well as significant loss of adhesive strength when exposed to moisture and ionic compounds, such as sweat. To address these common issues, the development of a polyelectrolyte\u2010based skin adhesive for wearable devices is underway. Here, it is demonstrated how coacervation is induced with a system composed of polyethylenimine (PEI) and sodium hexametaphosphate (PSP) as the counter polyelectrolyte. The coacervate is deposited onto a polyurethane film to form an effective adhesive that is mechanically comparable to a commercially available one, offering a promising alternative for wearable devices.<\/jats:p>","DOI":"10.1002\/marc.202500117","type":"journal-article","created":{"date-parts":[[2025,4,17]],"date-time":"2025-04-17T06:46:07Z","timestamp":1744872367000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":3,"title":["Polyelectrolyte Complex Coacervate Adhesive for Wearable Medical Devices"],"prefix":"10.1002","volume":"46","author":[{"given":"Maya D.","family":"Montemayor","sequence":"first","affiliation":[{"name":"Department of Chemistry College Station Texas A&amp;M University  TX 77843 USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-9231-6058","authenticated-orcid":false,"given":"Ethan T.","family":"Iverson","sequence":"additional","affiliation":[{"name":"Department of Chemistry College Station Texas A&amp;M University  TX 77843 USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Landon R.","family":"Dahle","sequence":"additional","affiliation":[{"name":"Department of Biomedical Engineering College Station Texas A&amp;M University  TX 77843 USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Amy","family":"Green","sequence":"additional","affiliation":[{"name":"Department of Biomedical Engineering College Station Texas A&amp;M University  TX 77843 USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Elizabeth","family":"Tenorio","sequence":"additional","affiliation":[{"name":"Department of Biomedical Engineering College Station Texas A&amp;M University  TX 77843 USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Alexandra V.","family":"Moran","sequence":"additional","affiliation":[{"name":"Department of Materials Science &amp; Engineering and Mechanical Engineering College Station Texas A&amp;M University  TX 77843 USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Danixa","family":"Rodriguez\u2010Melendez","sequence":"additional","affiliation":[{"name":"Department of Chemistry College Station Texas A&amp;M University  TX 77843 USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Edward","family":"Chang","sequence":"additional","affiliation":[{"name":"Department of Materials Science &amp; Engineering and Mechanical Engineering College Station Texas A&amp;M University  TX 77843 USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0009-2697-0981","authenticated-orcid":false,"given":"Margaret J.","family":"Karim","sequence":"additional","affiliation":[{"name":"Department of Chemistry College Station Texas A&amp;M University  TX 77843 USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Balakrishna","family":"Haridas","sequence":"additional","affiliation":[{"name":"Department of Biomedical Engineering College Station Texas A&amp;M University  TX 77843 USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-5241-9741","authenticated-orcid":false,"given":"Jaime C.","family":"Grunlan","sequence":"additional","affiliation":[{"name":"Department of Chemistry College Station Texas A&amp;M University  TX 77843 USA"},{"name":"Department of Materials Science &amp; Engineering and Mechanical Engineering College Station Texas A&amp;M University  TX 77843 USA"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2025,4,17]]},"reference":[{"key":"e_1_2_7_1_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41528-021-00107-x"},{"key":"e_1_2_7_2_1","doi-asserted-by":"publisher","DOI":"10.1177\/1932296814529893"},{"key":"e_1_2_7_3_1","doi-asserted-by":"publisher","DOI":"10.1111\/cod.12866"},{"key":"e_1_2_7_4_1","doi-asserted-by":"publisher","DOI":"10.1111\/cod.12647"},{"key":"e_1_2_7_5_1","doi-asserted-by":"publisher","DOI":"10.1111\/cod.13044"},{"key":"e_1_2_7_6_1","doi-asserted-by":"publisher","DOI":"10.1177\/1932296818762946"},{"key":"e_1_2_7_7_1","doi-asserted-by":"publisher","DOI":"10.1111\/cod.12995"},{"key":"e_1_2_7_8_1","doi-asserted-by":"publisher","DOI":"10.1097\/DER.0000000000000575"},{"key":"e_1_2_7_9_1","doi-asserted-by":"publisher","DOI":"10.1111\/cod.13012"},{"key":"e_1_2_7_10_1","doi-asserted-by":"publisher","DOI":"10.1002\/adhm.201800275"},{"key":"e_1_2_7_11_1","doi-asserted-by":"publisher","DOI":"10.12968\/jowc.2020.29.Sup3c.S1"},{"key":"e_1_2_7_12_1","author":"Kwant A. 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