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Herein, a polyester (PET) fabric covered with a vertically aligned 3D tower\u2010like ferrosoferric oxide (Fe<jats:sub>3<\/jats:sub>O<jats:sub>4<\/jats:sub>) array via a convenient magnetically driven spray\u2010coating method is reported, and both the spatial density and height of the Fe<jats:sub>3<\/jats:sub>O<jats:sub>4<\/jats:sub> array are tunable upon spraying time. It shows an extremely high solar absorbance (98.6%) in the entire solar spectrum, which is superior to the corresponding 2D Fe<jats:sub>3<\/jats:sub>O<jats:sub>4<\/jats:sub> structure (91.1%). Combining the obtained 3D Fe<jats:sub>3<\/jats:sub>O<jats:sub>4<\/jats:sub>\/PET with a yolk\u2010shell hydrophobic\/superhydrophilic modified melamine\u2010formaldehyde (mMF) sponge, the carefully designed and fabricated 3D Fe<jats:sub>3<\/jats:sub>O<jats:sub>4<\/jats:sub>\/PET\u2010mMF evaporator can realize a high water evaporation rate of 1.59\u00a0kg m<jats:sup>\u22122<\/jats:sup> h<jats:sup>\u22121<\/jats:sup> under 1\u00a0kW m<jats:sup>\u22122<\/jats:sup> solar illumination, outperforming most related solar steam generation systems. With the advantages of cost\u2010effectiveness, high evaporation rate, reliable endurance, and structural controllability, this 3D structural design provides an avenue to build up high\u2010performance solar energy\u2010driven water steam generation systems.<\/jats:p>","DOI":"10.1002\/smll.202105198","type":"journal-article","created":{"date-parts":[[2021,11,26]],"date-time":"2021-11-26T11:21:57Z","timestamp":1637925717000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":48,"title":["Magnetically Driven Tunable 3D Structured Fe<sub>3<\/sub>O<sub>4<\/sub> Vertical Array for High\u2010Performance Solar Steam Generation"],"prefix":"10.1002","volume":"18","author":[{"given":"Xiangyi","family":"Zhang","sequence":"first","affiliation":[{"name":"School of Materials Science and Engineering Wuhan Textile University  Wuhan 430200 P. R. 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