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However, the non\u2010adjustability pore size of traditional membranes limits the application of ion capture due to their low selectivity for target ions. Recently, covalent organic frameworks (COFs) have become a promising candidate for construction of advanced ion separation membranes for ion resource recovery due to their low density, large surface area, tunable channel structure, and tailored functionality. This tutorial review aims to analyze and summarize the progress in understanding ion capture mechanisms, preparation processes, and applications of COF\u2010based membranes. First, the design principles for target ion selectivity are illustrated in terms of theoretical simulation of ions transport in COFs, and key properties for ion selectivity of COFs and COF\u2010based membranes. Next, the fabrication methods of diverse COF\u2010based membranes are classified into pure COF membranes, COF continuous membranes, and COF mixed matrix membranes. Finally, current applications of COF\u2010based membranes are highlighted: desalination, extraction, removal of toxic metal ions, radionuclides and lithium, and acid recovery. This review presents promising approaches for design, preparation, and application of COF\u2010based membranes in ion selectivity for recovery of ionic resources.<\/jats:p>","DOI":"10.1002\/smll.202206041","type":"journal-article","created":{"date-parts":[[2022,11,30]],"date-time":"2022-11-30T06:06:22Z","timestamp":1669788382000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":43,"title":["Advanced Covalent Organic Framework\u2010Based Membranes for Recovery of Ionic Resources"],"prefix":"10.1002","volume":"19","author":[{"ORCID":"https:\/\/orcid.org\/0000-0003-2861-6379","authenticated-orcid":false,"given":"Chao","family":"Wu","sequence":"first","affiliation":[{"name":"Department of Chemical Engineering KU Leuven  Celestijnenlaan 200F Leuven B\u20103001 Belgium"},{"name":"Department of Environmental Science and Engineering Tongji University  1239 Siping Road Shanghai 200092 P. R. 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