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Owing to the special microenvironment of neural tissues and biological characteristics of neural cells, a considerable number of neurological disorders are currently incurable. In the past few years, the development of nanoplatforms based on metal\u2013organic frameworks (MOFs) has broadened opportunities for offering sensitive diagnosis\/monitoring and effective therapy of neurology\u2010related diseases. In this article, the obstacles for neurotherapeutics, including delayed diagnosis and misdiagnosis, the existence of blood brain barrier (BBB), off\u2010target treatment, irrepressible inflammatory storm\/oxidative stress, and irreversible nerve cell death are summarized. Correspondingly, MOFs\u2010based diagnostic\/monitoring strategies such as neuroimaging and biosensors (electrochemistry, fluorometry, colorimetry, electrochemiluminescence, etc.) and MOFs\u2010based therapeutic strategies including higher BBB permeability, targeting specific lesion sites, attenuation of neuroinflammation\/oxidative stress as well as regeneration of nerve cells, are extensively highlighted for the management of neurological diseases. Finally, the challenges of the present research from perspective of clinical translation are discussed, hoping to facilitate interdisciplinary studies at the intersections between MOFs\u2010based nanoplatforms and neurotheranostics.<\/jats:p>","DOI":"10.1002\/smll.202206575","type":"journal-article","created":{"date-parts":[[2023,3,13]],"date-time":"2023-03-13T05:37:45Z","timestamp":1678685865000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":32,"title":["Metal\u2013Organic Frameworks\u2010Based Nanoplatforms for the Theranostic Applications of Neurological Diseases"],"prefix":"10.1002","volume":"19","author":[{"given":"Huicong","family":"Niu","sequence":"first","affiliation":[{"name":"Department of Neurology Minhang Hospital Fudan University  Shanghai 200032 P. R. China"},{"name":"State Key Laboratory of High Performance Ceramics and Superfine Microstructure Shanghai Institute of Ceramics Chinese Academy of Sciences  Shanghai 200050 P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Hui","family":"Bu","sequence":"additional","affiliation":[{"name":"The Second Hospital of Hebei Medical University  Shijiazhuang 050000 P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jing","family":"Zhao","sequence":"additional","affiliation":[{"name":"Department of Neurology Minhang Hospital Fudan University  Shanghai 200032 P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-9031-8861","authenticated-orcid":false,"given":"Yufang","family":"Zhu","sequence":"additional","affiliation":[{"name":"State Key Laboratory of High Performance Ceramics and Superfine Microstructure Shanghai Institute of Ceramics Chinese Academy of Sciences  Shanghai 200050 P. R. 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