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As an alternative to traditional antibiotics, nanozymes attract more and more attention from the scientific researchers in recent years. Developing nanozymes\u2010based antibacterial materials opens up a new avenue for the bacterial disinfection and sterilization. In this review, the classification of nanozymes and their antibacterial mechanisms are discussed. The surface and composition of nanozymes are critical for the antibacterial efficacy, which can be tailored to enhance both the bacterial binding and the antibacterial activity. On the one hand, the surface modification of nanozymes enables binding and targeting of bacteria that improves the antibacterial performance of nanozymes including the biochemical recognition, the surface charge, and the surface topography. On the other hand, the composition of nanozymes can be modulated to achieve enhanced antibacterial performance including the single nanozyme\u2010mediated synergistic and multiple nanozymes\u2010mediated cascade catalytic antibacterial applications. In addition, the current challenges and future prospects of tailoring nanozymes for antibacterial applications are discussed. This review can provide insights into the design of future nanozymes\u2010based materials for the antibacterial treatments.<\/jats:p>","DOI":"10.1002\/smll.202302640","type":"journal-article","created":{"date-parts":[[2023,6,16]],"date-time":"2023-06-16T03:09:34Z","timestamp":1686884974000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":115,"title":["Tailoring the Surface and Composition of Nanozymes for Enhanced Bacterial Binding and Antibacterial Activity"],"prefix":"10.1002","volume":"19","author":[{"given":"Jinjie","family":"Hou","sequence":"first","affiliation":[{"name":"State Key Laboratory of Fluid Power and Mechatronic Systems College of Biosystems Engineering and Food Science Zhejiang University  Hangzhou 310058 P. R. 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