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To achieve this, a fully flexible and omni\u2010healable all\u2010hydrogel, that is dynamically crosslinked PVA@PANI hydrogel, is rationally designed and constructed via aniline\/DMSO\u2010emulsion\u2010templated in situ freezing\u2010polymerization strategy. The PVA@PANI sheet, not only possesses a honeycombed porous conductive mesh configuration with superior flexibility that provides numerous channels for unimpeded ions\/electron transport and maximizes the utilization efficiency of pseudocapacitive PANI, but also can conform to complicated body surface, enabling effective detection and discrimination of body movements. As a consequence, the fabricated flexible PVA@PANI sheet electrode demonstrates an unprecedented specific capacitance (936.8\u00a0F\u00a0g<jats:sup>\u22121<\/jats:sup>) and the assembled symmetric flexible all\u2010solid\u2010state supercapacitor delivers an extraordinary energy density of 40.98\u00a0Wh\u00a0kg<jats:sup>\u22121<\/jats:sup>, outperforming the previously highest\u2010reported values of stretchable PVA@PANI hydrogel\u2010based supercapacitors. What is more, such a flexible supercapacitor electrode enables precisely monitoring the full\u2010range human activities in real\u2010time, and fulfilling a quick response and excellent self\u2010recovery. These outstanding flexible sensing and energy storage performances render this emerging PVA@PANI hydrogel highly promising for the next\u2010generation wearable self\u2010powered sensing electronics.<\/jats:p>","DOI":"10.1002\/smll.202305448","type":"journal-article","created":{"date-parts":[[2023,10,26]],"date-time":"2023-10-26T04:46:00Z","timestamp":1698295560000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":65,"title":["Dynamically Cross\u2010Linked, Self\u2010Healable, and Stretchable All\u2010Hydrogel Supercapacitor with Extraordinary Energy Density and Real\u2010Time Pressure Sensing"],"prefix":"10.1002","volume":"20","author":[{"given":"Muchun","family":"Xu","sequence":"first","affiliation":[{"name":"Yunnan Key Laboratory of Electromagnetic Materials and Devices National Center for International Research on Photoelectric and Energy Materials School of Materials and Energy Yunnan University  Kunming 650091 P. R. 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