{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,9,13]],"date-time":"2026-09-13T01:36:44Z","timestamp":1789263404313,"version":"build-2803163510"},"reference-count":52,"publisher":"Wiley","issue":"6","license":[{"start":{"date-parts":[[2023,9,29]],"date-time":"2023-09-29T00:00:00Z","timestamp":1695945600000},"content-version":"vor","delay-in-days":0,"URL":"http:\/\/onlinelibrary.wiley.com\/termsAndConditions#vor"}],"funder":[{"DOI":"10.13039\/501100004826","name":"Natural Science Foundation of Beijing Municipality","doi-asserted-by":"publisher","award":["2192044"],"award-info":[{"award-number":["2192044"]}],"id":[{"id":"10.13039\/501100004826","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100012226","name":"Fundamental Research Funds for the Central Universities","doi-asserted-by":"publisher","award":["XK1802\u20102"],"award-info":[{"award-number":["XK1802\u20102"]}],"id":[{"id":"10.13039\/501100012226","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":["onlinelibrary.wiley.com"],"crossmark-restriction":true},"short-container-title":["Small"],"published-print":{"date-parts":[[2024,2]]},"abstract":"<jats:title>Abstract<\/jats:title><jats:p>Microwave absorbers with high efficiency and mechanical robustness are urgently desired to cope with more complex and harsh application scenarios. However, manipulating the trade\u2010off between microwave absorption performance and mechanical properties is seldom realized in microwave absorbers. Here, a chemistry\u2010tailored charge dynamic engineering strategy is proposed for sparking hetero\u2010interfacial polarization and thus coordinating microwave attenuation ability with the interfacial bonding, endowing polymer\u2010based composites with microwave absorption efficiency and mechanical toughness. The absorber designed by this new conceptual approach exhibits remarkable Ku\u2010band microwave absorption efficiency (\u221255.3\u00a0dB at a thickness of 1.5\u00a0mm) and satisfactory effective absorption bandwidth (5.0\u00a0GHz) as well as desirable interfacial shear strength (97.5\u00a0MPa). The calculated differential charge density depicts the uneven distribution of space charge and the intense hetero\u2010interfacial polarization, clarifying the structure\u2013performance relationship from a theoretical perspective. This work breaks through traditional single performance\u2010oriented design methods and ushers a new direction for next\u2010generation microwave absorbers.<\/jats:p>","DOI":"10.1002\/smll.202306104","type":"journal-article","created":{"date-parts":[[2023,9,30]],"date-time":"2023-09-30T04:43:31Z","timestamp":1696049011000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":23,"title":["Charge Dynamics Engineering Sparks Hetero\u2010Interfacial Polarization for an Ultra\u2010Efficient Microwave Absorber with Mechanical Robustness"],"prefix":"10.1002","volume":"20","author":[{"given":"Xianhua","family":"Huan","sequence":"first","affiliation":[{"name":"School of Electrical Engineering and Automation Hefei University of Technology  Hefei 230009 P. R. China"},{"name":"State Key Laboratory of Organic\u2013Inorganic Composites Key Laboratory of Carbon Fibre and Functional Polymer Ministry of Education College of Materials Science and Engineering Beijing University of Chemical Technology  Beijing 100029 P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Hefeng","family":"Li","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Organic\u2013Inorganic Composites Key Laboratory of Carbon Fibre and Functional Polymer Ministry of Education College of Materials Science and Engineering Beijing University of Chemical Technology  Beijing 100029 P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yuxiao","family":"Song","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Organic\u2013Inorganic Composites Key Laboratory of Carbon Fibre and Functional Polymer Ministry of Education College of Materials Science and Engineering Beijing University of Chemical Technology  Beijing 100029 P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jintao","family":"Luo","sequence":"additional","affiliation":[{"name":"Beijing Spacecraft Manufacturing Factory Co. Ltd.  Beijing 100094 P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Cong","family":"Liu","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Organic\u2013Inorganic Composites Key Laboratory of Carbon Fibre and Functional Polymer Ministry of Education College of Materials Science and Engineering Beijing University of Chemical Technology  Beijing 100029 P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Ke","family":"Xu","sequence":"additional","affiliation":[{"name":"Inner Mongolia Aerospace Hong Gang Machinery Corporation Limited  Inner Mongolia 010076 P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Hongbo","family":"Geng","sequence":"additional","affiliation":[{"name":"Inner Mongolia Aerospace Hong Gang Machinery Corporation Limited  Inner Mongolia 010076 P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xiaodong","family":"Guo","sequence":"additional","affiliation":[{"name":"Inner Mongolia Aerospace Hong Gang Machinery Corporation Limited  Inner Mongolia 010076 P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Chen","family":"Chen","sequence":"additional","affiliation":[{"name":"Xi'an Institute of Aerospace Propulsion Technology  Xi'an 710025 P. R. China"},{"name":"The 41st Institute of the Fourth Academy of CSAC National Key Lab of Combustion Flow and Thermo\u2010structure  Xi'an 710025 P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Lei","family":"Zu","sequence":"additional","affiliation":[{"name":"School of Mechanical Engineering Hefei University of Technology  Hefei 230000 P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-9687-6872","authenticated-orcid":false,"given":"Xiaolong","family":"Jia","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Organic\u2013Inorganic Composites Key Laboratory of Carbon Fibre and Functional Polymer Ministry of Education College of Materials Science and Engineering Beijing University of Chemical Technology  Beijing 100029 P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jisheng","family":"Zhou","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Organic\u2013Inorganic Composites Key Laboratory of Carbon Fibre and Functional Polymer Ministry of Education College of Materials Science and Engineering Beijing University of Chemical Technology  Beijing 100029 P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Haobin","family":"Zhang","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Organic\u2013Inorganic Composites Key Laboratory of Carbon Fibre and Functional Polymer Ministry of Education College of Materials Science and Engineering Beijing University of Chemical Technology  Beijing 100029 P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xiaoping","family":"Yang","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Organic\u2013Inorganic Composites Key Laboratory of Carbon Fibre and Functional Polymer Ministry of Education College of Materials Science and Engineering Beijing University of Chemical Technology  Beijing 100029 P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2023,9,29]]},"reference":[{"key":"e_1_2_8_1_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.pmatsci.2023.101088"},{"key":"e_1_2_8_2_1","doi-asserted-by":"publisher","DOI":"10.1002\/adma.202107538"},{"key":"e_1_2_8_3_1","doi-asserted-by":"publisher","DOI":"10.1002\/adma.202002112"},{"key":"e_1_2_8_4_1","doi-asserted-by":"publisher","DOI":"10.1002\/adma.202106195"},{"key":"e_1_2_8_5_1","doi-asserted-by":"publisher","DOI":"10.1002\/adfm.202111045"},{"key":"e_1_2_8_6_1","doi-asserted-by":"publisher","DOI":"10.1021\/acsanm.0c01981"},{"key":"e_1_2_8_7_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.carbon.2023.118036"},{"key":"e_1_2_8_8_1","doi-asserted-by":"publisher","DOI":"10.1002\/smll.202106302"},{"key":"e_1_2_8_9_1","doi-asserted-by":"publisher","DOI":"10.1002\/smll.202105411"},{"key":"e_1_2_8_10_1","doi-asserted-by":"publisher","DOI":"10.1002\/adfm.202209898"},{"key":"e_1_2_8_11_1","doi-asserted-by":"publisher","DOI":"10.1002\/adfm.202204591"},{"key":"e_1_2_8_12_1","doi-asserted-by":"publisher","DOI":"10.1126\/science.aba7977"},{"key":"e_1_2_8_13_1","doi-asserted-by":"publisher","DOI":"10.1021\/acsami.9b00593"},{"key":"e_1_2_8_14_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.jcis.2019.08.020"},{"key":"e_1_2_8_15_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.jmst.2022.09.050"},{"key":"e_1_2_8_16_1","doi-asserted-by":"publisher","DOI":"10.1021\/acsami.1c06446"},{"key":"e_1_2_8_17_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.compositesb.2021.109173"},{"key":"e_1_2_8_18_1","author":"Chen G.","year":"2023","journal-title":"Adv. Mater."},{"key":"e_1_2_8_19_1","doi-asserted-by":"publisher","DOI":"10.1002\/adfm.202106677"},{"key":"e_1_2_8_20_1","doi-asserted-by":"publisher","DOI":"10.1002\/adfm.202100470"},{"key":"e_1_2_8_21_1","doi-asserted-by":"publisher","DOI":"10.1002\/adfm.202002595"},{"key":"e_1_2_8_22_1","doi-asserted-by":"publisher","DOI":"10.1002\/adfm.202202588"},{"key":"e_1_2_8_23_1","doi-asserted-by":"publisher","DOI":"10.1002\/adma.201603009"},{"key":"e_1_2_8_24_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.compositesb.2020.107987"},{"key":"e_1_2_8_25_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.compositesb.2021.108656"},{"key":"e_1_2_8_26_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.cej.2019.122860"},{"key":"e_1_2_8_27_1","doi-asserted-by":"publisher","DOI":"10.1002\/smll.201900900"},{"key":"e_1_2_8_28_1","doi-asserted-by":"publisher","DOI":"10.1021\/acsami.6b07555"},{"key":"e_1_2_8_29_1","doi-asserted-by":"publisher","DOI":"10.1002\/adfm.200900011"},{"key":"e_1_2_8_30_1","doi-asserted-by":"publisher","DOI":"10.1002\/smll.201800987"},{"key":"e_1_2_8_31_1","doi-asserted-by":"publisher","DOI":"10.1002\/adma.201907156"},{"key":"e_1_2_8_32_1","doi-asserted-by":"publisher","DOI":"10.1002\/adma.202105067"},{"key":"e_1_2_8_33_1","doi-asserted-by":"publisher","DOI":"10.1002\/anie.202216286"},{"key":"e_1_2_8_34_1","doi-asserted-by":"publisher","DOI":"10.1109\/TDEI.2022.3221384"},{"key":"e_1_2_8_35_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41467-021-24511-z"},{"key":"e_1_2_8_36_1","doi-asserted-by":"publisher","DOI":"10.1021\/nl050788p"},{"key":"e_1_2_8_37_1","doi-asserted-by":"publisher","DOI":"10.1002\/adfm.200304434"},{"key":"e_1_2_8_38_1","doi-asserted-by":"publisher","DOI":"10.1002\/smll.201203135"},{"key":"e_1_2_8_39_1","doi-asserted-by":"publisher","DOI":"10.1002\/smll.202001686"},{"key":"e_1_2_8_40_1","doi-asserted-by":"publisher","DOI":"10.1021\/acsami.1c04991"},{"key":"e_1_2_8_41_1","doi-asserted-by":"publisher","DOI":"10.1002\/adfm.201807398"},{"key":"e_1_2_8_42_1","volume-title":"Basic Electromagnetism and Materials","author":"Moliton A.","year":"2007"},{"key":"e_1_2_8_43_1","doi-asserted-by":"publisher","DOI":"10.1039\/c2jm33124a"},{"key":"e_1_2_8_44_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.jmat.2021.02.017"},{"key":"e_1_2_8_45_1","doi-asserted-by":"publisher","DOI":"10.1002\/advs.202105553"},{"key":"e_1_2_8_46_1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevB.70.144106"},{"key":"e_1_2_8_47_1","doi-asserted-by":"publisher","DOI":"10.1063\/1.1290691"},{"key":"e_1_2_8_48_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.carbon.2017.12.026"},{"key":"e_1_2_8_49_1","doi-asserted-by":"publisher","DOI":"10.1002\/aenm.201803951"},{"key":"e_1_2_8_50_1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevB.99.085429"},{"key":"e_1_2_8_51_1","doi-asserted-by":"publisher","DOI":"10.1021\/acsami.1c14535"},{"key":"e_1_2_8_52_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.cej.2020.124255"}],"container-title":["Small"],"original-title":[],"language":"en","link":[{"URL":"https:\/\/onlinelibrary.wiley.com\/doi\/pdf\/10.1002\/smll.202306104","content-type":"unspecified","content-version":"vor","intended-application":"similarity-checking"}],"deposited":{"date-parts":[[2024,3,14]],"date-time":"2024-03-14T13:56:18Z","timestamp":1710424578000},"score":1,"resource":{"primary":{"URL":"https:\/\/onlinelibrary.wiley.com\/doi\/10.1002\/smll.202306104"}},"subtitle":[],"short-title":[],"issued":{"date-parts":[[2023,9,29]]},"references-count":52,"journal-issue":{"issue":"6","published-print":{"date-parts":[[2024,2]]}},"alternative-id":["10.1002\/smll.202306104"],"URL":"https:\/\/doi.org\/10.1002\/smll.202306104","archive":["Portico"],"relation":{},"ISSN":["1613-6810","1613-6829"],"issn-type":[{"value":"1613-6810","type":"print"},{"value":"1613-6829","type":"electronic"}],"subject":[],"published":{"date-parts":[[2023,9,29]]},"assertion":[{"value":"2023-07-20","order":0,"name":"received","label":"Received","group":{"name":"publication_history","label":"Publication History"}},{"value":"2023-09-29","order":2,"name":"published","label":"Published","group":{"name":"publication_history","label":"Publication History"}}],"article-number":"2306104"}}