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Violet phosphorus (VP) as a new allotrope of available phosphorus with outstanding electro\u2010optical properties and stability has attracted more and more attention in the past several years. In this study, large\u2010scale, high\u2010yield VP microfiber vertical arrays have been successfully developed on a Sn\u2010coated graphite paper and are used as the memristor functional layers to build reliable, low\u2010power artificial synaptic devices. The VP devices can well mimic the major synaptic functions such as short\u2010term memory (STM), long\u2010term memory (LTM), paired\u2010pulse facilitation (PPF), spike timing\u2010dependent plasticity (STDP), and spike rate\u2010dependent plasticity (SRDP) under both electrical and light stimulation conditions, even the dendritic synapse functions and simple logical operations. By virtue of the excellent performance, the VP artificial synapse devices can be conductive to building high\u2010performance optic\u2010neural synaptic devices simulating the human\u2010like optic nerve system. On this basis, Pavlov's associative memory can be successfully implemented optically. This study provides a promising approach for the design and manufacture of VP\u2010based artificial synaptic devices and outlines a direction with multifunctional neural devices.<\/jats:p>","DOI":"10.1002\/smll.202306998","type":"journal-article","created":{"date-parts":[[2023,11,15]],"date-time":"2023-11-15T04:00:53Z","timestamp":1700020853000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":29,"title":["Artificial Optoelectronic Synapse Based on Violet Phosphorus Microfiber Arrays"],"prefix":"10.1002","volume":"20","author":[{"given":"Liyan","family":"Dong","sequence":"first","affiliation":[{"name":"Materials Institute of Atomic and Molecular Science Shaanxi University of Science and Technology  Xi'an 710021 P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Shuai","family":"Yuan","sequence":"additional","affiliation":[{"name":"Materials Institute of Atomic and Molecular Science Shaanxi University of Science and Technology  Xi'an 710021 P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Guodong","family":"Wei","sequence":"additional","affiliation":[{"name":"Materials Institute of Atomic and Molecular Science Shaanxi University of Science and Technology  Xi'an 710021 P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Peifen","family":"Zhu","sequence":"additional","affiliation":[{"name":"Department of Electrical Engineering and Computer Science University of Missouri  Columbia MO 65211 USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Shufang","family":"Ma","sequence":"additional","affiliation":[{"name":"Materials Institute of Atomic and Molecular Science Shaanxi University of Science and Technology  Xi'an 710021 P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Bingshe","family":"Xu","sequence":"additional","affiliation":[{"name":"Materials Institute of Atomic and Molecular Science Shaanxi University of Science and Technology  Xi'an 710021 P. R. China"},{"name":"Shanxi\u2010Zheda Institute of Advanced Materials and Chemical Engineering  Taiyuan 030024 P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-0168-2974","authenticated-orcid":false,"given":"Ya","family":"Yang","sequence":"additional","affiliation":[{"name":"CAS Center for Excellence in Nanoscience, Beijing Key Laboratory of Micro\u2010nano Energy and Sensor, Beijing Institute of Nanoenergy and Nanosystems Chinese Academy of Sciences  Beijing 101400 P. R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2023,11,14]]},"reference":[{"key":"e_1_2_8_1_1","unstructured":"C. D.Schuman T. E.Potok R. M.Patton J. D.Birdwell M. E.Dean G. S.Rose J. 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