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Once the superhydrophobic surface is damaged underwater, water seeps into gaps among micro\/nano structures. The air film diffuses into water and eventually disappears during immersion without actively replenishing the gas, which results in the impossible of self\u2010healing. Here, an underwater self\u2010healing superhydrophobic coating with the synergetic effect of hydrogen bonds and self\u2010formed bubbles via the spraying method is fabricated. The movement of hydrogen bonds of the prepared polyurethane enables microstructures to reconstruct at room temperature and self\u2010formed bubbles of effervescent materials underwater actively replenish gas before microstructures completely self\u2010healing, achieving the self\u2010healing property of the superhydrophobic coating. Moreover, the hydrophilic effervescent material is sprayed along with unmodified micron\u2010scaled particles because modified nano\u2010scale particles are key factors for the realization of superhydrophobic coating. An underwater stable superhydrophobic surface with pressure resistance (4.9\u00a0kPa) is demonstrated. This superhydrophobic coating also shows excellent drag reduction, anti\u2010icing, and anti\u2010corrosion properties. This facile and scalable method offers a new route that an underwater self\u2010healing superhydrophobic coating executes the gas film recovery.<\/jats:p>","DOI":"10.1002\/smll.202309012","type":"journal-article","created":{"date-parts":[[2024,1,5]],"date-time":"2024-01-05T02:16:09Z","timestamp":1704420969000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":57,"title":["Underwater Bionic Self\u2010Healing Superhydrophobic Coating with the Synergetic Effect Of Hydrogen Bonds and Self\u2010Formed Bubbles"],"prefix":"10.1002","volume":"20","author":[{"ORCID":"https:\/\/orcid.org\/0000-0001-7923-5950","authenticated-orcid":false,"given":"Hao","family":"Li","sequence":"first","affiliation":[{"name":"School of Material Science and Engineering Shandong University of Science and Technology  Qingdao 266590 P.R. 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