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Herein, inspired by the glass\u2010blowing art, a spontaneous, controllable, and scalable strategy is proposed to prepare hollow carbon materials by inner blowing and outside blocking. Specifically, hierarchically neuron\u2010like hollow carbon materials (HCMSs) with various sizes are fabricated from melamine\u2010formaldehyde sponge (MS) waste. Benefiting from the synergistic of the hollow \u201ccell body\u201d and the connected \u201cprotrusions\u201d networks, HCMSs reveal superior electromagnetic absorption performance with a strong reflection loss of \u221254.9\u00a0dB, electromagnetic\u2010heat conversion ability with a high conversion efficiency of 34.4%, and efficient energy storage performance in supercapacitor. Furthermore, a multifunctional device integrating electromagnetic\u2010heat\u2010electrical energy conversion is designed, and its feasibility is proved by experiments and theoretical calculations. The integrated device reveals an output voltage of 34.5\u00a0mV and a maximum output power of 0.89 \u00b5W with electromagnetic radiation for 60\u00a0s. This work provides a novel solution to recycle polymer waste, electromagnetic energy, and unwanted thermal energy.<\/jats:p>","DOI":"10.1002\/smll.202401995","type":"journal-article","created":{"date-parts":[[2024,5,31]],"date-time":"2024-05-31T04:39:47Z","timestamp":1717130387000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":21,"title":["Glass\u2010Blowing\u2010Inspired Upcycling of Thermosetting Polymer to Neuron\u2010Like Hierarchical Carbon for Microwave Absorption and Conversion"],"prefix":"10.1002","volume":"20","author":[{"given":"Yang\u2010Yang","family":"Xie","sequence":"first","affiliation":[{"name":"The Collaborative Innovation Center for Eco\u2010Friendly and Fire\u2010Safety Polymeric Materials (MoE) National Engineering Laboratory of Eco\u2010Friendly Polymeric Materials (Sichuan) State Key Laboratory of Polymer Materials Engineering College of Chemistry Sichuan University  Chengdu 610064 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