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One of the key issues affecting the development of nuclear energy is how to make full use of depleted uranium resources efficiently. Here, U element with unique coordination mode of 5f electron is spacer bonded to transition metal with 3d orbit through the adsorption and anchoring effect of MXene, thus U and Co dual doped MXene catalyst is constructed along with the comprehensive utilization of depleted uranium resources. The as\u2010prepared U\u2010Co\/MXene catalyst demonstrates excellent overpotential of only 184\u00a0mV at \u221210\u00a0mA cm\n                    <jats:sup>\u22122<\/jats:sup>\n                    and excellent stability up to 150\u00a0h, significantly surpassing the bare MXene substrate. Theoretical calculations indicate that the U and Co dual doping optimizes the electronic structure of MXene catalyst by forming the U\u2010O\u2010Co network, thereby improving the thermodynamics of H\n                    <jats:sup>*<\/jats:sup>\n                    adsorption during the catalytic transition state. This research opens up a new path for the recovery of depleted uranium resources and the development of functional actinide catalysts.\n                  <\/jats:p>","DOI":"10.1002\/smll.202402847","type":"journal-article","created":{"date-parts":[[2024,6,7]],"date-time":"2024-06-07T03:41:35Z","timestamp":1717731695000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":27,"title":["U and Co Dual Single\u2010Atom Doped MXene for Accelerating Electrocatalytic Hydrogen Evolution Activity"],"prefix":"10.1002","volume":"20","author":[{"given":"Yanze","family":"Wu","sequence":"first","affiliation":[{"name":"Laboratory of Nuclear Energy Chemistry Institute of High Energy Physics Chinese Academy of Sciences  Beijing 100049 China"},{"name":"Spallation Neutron Source Science Center  Dongguan 523803 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