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Consequently, their fabrication is dominated by methods of direct material manipulation, which struggle to meet the designers\u2019 demands regarding resolution, material freedom, production time, and cost. A two\u2010step, computer\u2010controlled is presented, multi\u2010material self\u2010assembly technique that allows heterogenous patterns of several centimeters with features down to 12.5\u00a0\u00b5m in size. First, a micro plasma jet selectively programs the surface energy of a polydimethylsiloxane substrate through localized chemical functionalization. Second, polar fluids containing functional materials are simplistically introduced which then self\u2010assemble according to the patterned regions of high surface energy over timescales of the order of seconds. In\u2010process control enables both high\u2010resolution patterning and high throughput. This approach is demonstrated to produce heterogenous patterns of materials with varying conductive, magnetic, and mechanical properties. These include magneto\u2010mechanical films and flexible electronic devices with unprecedented processing times and economy for high\u2010resolution patterns. This self\u2010assembly approach can disrupt the current lithography\/direct write paradigm that dominates micro\/meso\u2010fabrication, enabling the next generation of devices across a broad range of fields via a flexible, industrially scalable, and environmentally friendly manufacturing route.<\/jats:p>","DOI":"10.1002\/smll.202408822","type":"journal-article","created":{"date-parts":[[2024,12,30]],"date-time":"2024-12-30T03:56:22Z","timestamp":1735530982000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":6,"title":["High\u2010Resolution Self\u2010Assembly of Functional Materials and Microscale Devices via Selective Plasma Induced Surface Energy Programming"],"prefix":"10.1002","volume":"21","author":[{"ORCID":"https:\/\/orcid.org\/0000-0002-0854-8674","authenticated-orcid":false,"given":"Luke J.","family":"Tinsley","sequence":"first","affiliation":[{"name":"Future Manufacturing Processes Research Group, School of Mechanical Engineering University of Leeds  LS2 9JT United\u00a0Kingdom"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Prakash","family":"Karipoth","sequence":"additional","affiliation":[{"name":"Future Manufacturing Processes Research Group, School of Mechanical Engineering University of Leeds  LS2 9JT United\u00a0Kingdom"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"James H.","family":"Chandler","sequence":"additional","affiliation":[{"name":"STORM Lab, School of Electrical Engineering University of Leeds  LS2 9JT United\u00a0Kingdom"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Silvia","family":"Taccola","sequence":"additional","affiliation":[{"name":"Future Manufacturing Processes Research Group, School of Mechanical Engineering University of Leeds  LS2 9JT United\u00a0Kingdom"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Pietro","family":"Valdastri","sequence":"additional","affiliation":[{"name":"STORM Lab, School of Electrical Engineering University of Leeds  LS2 9JT United\u00a0Kingdom"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Russell A.","family":"Harris","sequence":"additional","affiliation":[{"name":"Future Manufacturing Processes Research Group, School of Mechanical Engineering University of Leeds  LS2 9JT United\u00a0Kingdom"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2024,12,29]]},"reference":[{"key":"e_1_2_10_1_1","doi-asserted-by":"publisher","DOI":"10.1126\/science.1070821"},{"key":"e_1_2_10_2_1","doi-asserted-by":"publisher","DOI":"10.1557\/mrs2005.208"},{"key":"e_1_2_10_3_1","doi-asserted-by":"publisher","DOI":"10.1049\/iet-nbt.2014.0020"},{"key":"e_1_2_10_4_1","doi-asserted-by":"publisher","DOI":"10.1002\/admt.201800692"},{"key":"e_1_2_10_5_1","doi-asserted-by":"publisher","DOI":"10.1002\/anie.201208397"},{"key":"e_1_2_10_6_1","doi-asserted-by":"publisher","DOI":"10.1038\/nature08016"},{"key":"e_1_2_10_7_1","doi-asserted-by":"publisher","DOI":"10.1038\/nnano.2012.189"},{"key":"e_1_2_10_8_1","doi-asserted-by":"publisher","DOI":"10.1126\/science.1962191"},{"key":"e_1_2_10_9_1","doi-asserted-by":"publisher","DOI":"10.1039\/C5SM00764J"},{"key":"e_1_2_10_10_1","doi-asserted-by":"publisher","DOI":"10.1109\/JMEMS.2010.2042681"},{"key":"e_1_2_10_11_1","doi-asserted-by":"publisher","DOI":"10.1073\/pnas.0500807102"},{"key":"e_1_2_10_12_1","volume":"36","author":"Cossio G.","year":"2024","journal-title":"Adv. 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