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Traditional PDES fabrication typically involves heating and extended processing time. In this study, a facile method where a solid\u2010solid mixture of lithium bis(trifluoromethane) sulfonimide (LiTFSI) and acrylamide (AAm) rapidly forms a PDES at room temperature, significantly simplifying the ionogel preparation is presented. By combining this PDES with\u00a0another\u00a0system,\u00a0comprising\u00a03\u2010[dimethyl\u2010[2\u2010(2\u2010methylprop\u20102\u2010enoyloxy)ethyl]azaniumyl]propane\u20101\u2010sulfonate (SBMA) and ethylene glycol (EG), an eutectic gel is successfully fabricated with exceptional mechanical and conductive properties. This gel exhibits a fracture stress of 0.8\u00a0MPa, fracture energy of 3.7\u00a0kJ m<jats:sup>\u22122<\/jats:sup>, adhesion strength of 60\u00a0kPa, transmittance over 90%, high conductivity (0.113 S m<jats:sup>\u22121<\/jats:sup>), and an outstanding temperature tolerance ranged from \u201050 to 50 \u00b0C. Notably, the absence of chemical crosslinkers and the presence of reversible interactions such as hydrogen bonding and ion\u2010dipole electrostatic forces impart excellent self\u2010healing capabilities. These combined features position the gel a promising candidate for multisensory ionic skins, capable of detecting pressure, temperature, humidity, and sweat. This work pioneers the rapid, mild\u2010condition synthesis of PDESs, paving the way for new techniques in ionic skin development.<\/jats:p>","DOI":"10.1002\/smll.202409754","type":"journal-article","created":{"date-parts":[[2024,12,2]],"date-time":"2024-12-02T05:04:47Z","timestamp":1733115887000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":30,"title":["Facile Preparation of Polymerizable Deep Eutectic Solvents Under Mild Conditions for Multisensory Ionic Skins"],"prefix":"10.1002","volume":"21","author":[{"given":"Menghan","family":"Pi","sequence":"first","affiliation":[{"name":"College of Polymer Science and Engineering, State Key Laboratory of Polymer Materials Engineering Sichuan University  Chengdu 610065 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Honglin","family":"Wu","sequence":"additional","affiliation":[{"name":"College of Polymer Science and Engineering, State Key Laboratory of Polymer Materials Engineering Sichuan University  Chengdu 610065 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Wenhao","family":"Li","sequence":"additional","affiliation":[{"name":"College of Polymer Science and Engineering, State Key Laboratory of Polymer Materials Engineering Sichuan University  Chengdu 610065 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Huanwei","family":"Shen","sequence":"additional","affiliation":[{"name":"College of Polymer Science and Engineering, State Key Laboratory of Polymer Materials Engineering Sichuan University  Chengdu 610065 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Min","family":"Li","sequence":"additional","affiliation":[{"name":"College of Polymer Science and Engineering, State Key Laboratory of Polymer Materials Engineering Sichuan University  Chengdu 610065 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-3449-8524","authenticated-orcid":false,"given":"Wei","family":"Cui","sequence":"additional","affiliation":[{"name":"College of Polymer Science and Engineering, State Key Laboratory of Polymer Materials Engineering Sichuan University  Chengdu 610065 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Rong","family":"Ran","sequence":"additional","affiliation":[{"name":"College of Polymer Science and Engineering, State Key Laboratory of Polymer Materials Engineering Sichuan University  Chengdu 610065 China"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2024,12]]},"reference":[{"key":"e_1_2_8_1_1","doi-asserted-by":"publisher","DOI":"10.1126\/science.abj9912"},{"key":"e_1_2_8_2_1","doi-asserted-by":"publisher","DOI":"10.1126\/sciadv.adh0615"},{"key":"e_1_2_8_3_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41467-024-45079-4"},{"key":"e_1_2_8_4_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41563-022-01195-4"},{"key":"e_1_2_8_5_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41467-022-30224-8"},{"key":"e_1_2_8_6_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41586-024-07564-0"},{"key":"e_1_2_8_7_1","doi-asserted-by":"publisher","DOI":"10.1002\/adma.202300114"},{"key":"e_1_2_8_8_1","doi-asserted-by":"publisher","DOI":"10.1039\/C8CS00325D"},{"key":"e_1_2_8_9_1","doi-asserted-by":"publisher","DOI":"10.1021\/acs.chemrev.0c00385"},{"key":"e_1_2_8_10_1","doi-asserted-by":"publisher","DOI":"10.1002\/adma.202309568"},{"key":"e_1_2_8_11_1","doi-asserted-by":"publisher","DOI":"10.1021\/acsenergylett.3c00340"},{"key":"e_1_2_8_12_1","doi-asserted-by":"publisher","DOI":"10.1002\/adma.202310102"},{"key":"e_1_2_8_13_1","doi-asserted-by":"publisher","DOI":"10.1002\/adfm.202408017"},{"key":"e_1_2_8_14_1","doi-asserted-by":"publisher","DOI":"10.1002\/adfm.202405130"},{"key":"e_1_2_8_15_1","doi-asserted-by":"publisher","DOI":"10.1002\/smll.202200421"},{"key":"e_1_2_8_16_1","doi-asserted-by":"publisher","DOI":"10.1002\/smll.202304828"},{"key":"e_1_2_8_17_1","doi-asserted-by":"publisher","DOI":"10.1002\/smtd.202100819"},{"key":"e_1_2_8_18_1","doi-asserted-by":"publisher","DOI":"10.1002\/adfm.202201846"},{"key":"e_1_2_8_19_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.nanoen.2022.107077"},{"key":"e_1_2_8_20_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.nanoen.2022.107284"},{"key":"e_1_2_8_21_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.nanoen.2022.107789"},{"key":"e_1_2_8_22_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.nanoen.2022.107442"},{"key":"e_1_2_8_23_1","doi-asserted-by":"publisher","DOI":"10.1002\/adma.202401151"},{"key":"e_1_2_8_24_1","volume":"62","author":"Li C.","year":"2023","journal-title":"Angew. 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