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However, the sluggish conversion kinetics between CO\u2082 and the discharge product lithium carbonate (Li\u2082CO\u2083) have hindered their practical applications. Herein, a flower\u2010like photosensitive metal\u2013organic framework (FJU\u2010115\u2010NS) has been employed as a cathodic electrocatalyst for Li\u2010CO\u2082 batteries. The FJU\u2010115\u2010NS with well\u2010ordered micropores and abundant exposed catalytic sites can effectively facilitate lithium ion transport and catalyze the Li\u2082CO\u2083 formation\/decomposition, leading to improved battery performance. At a current density of 200\u00a0mA g\u207b\u00b9, the FJU\u2010115\u2010NS battery exhibits a substantial discharge capacity of 31579.34\u00a0mA h g\u207b\u00b9, a low overpotential of 1.31\u00a0V, and stable operation over 3200 h. Importantly, under light irradiation, the charging voltage significantly dropped from 4.45\u00a0V (without light) to 3.43\u00a0V at a high current density of 2 A g\u207b\u00b9. Additionally, the cell demonstrated an exceptionally low overpotential of just 0.45\u00a0V at a current density of 200\u00a0mA g\u207b\u00b9, highlighting its enhanced efficiency under light\u2010assisted conditions. This work provides valuable guidance for developing light\u2010assisted MOF catalysts to upgrade the longevity and energy efficiency of Li\u2010CO\u2082 batteries.<\/jats:p>","DOI":"10.1002\/smll.202411559","type":"journal-article","created":{"date-parts":[[2025,1,31]],"date-time":"2025-01-31T03:59:56Z","timestamp":1738295996000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":23,"title":["MOF Nanosheet Enable Accelerated Redox Kinetics and Ultralow Overpotential for Light\u2010Assisted Li\u2010CO\n                    <sub>2<\/sub>\n                    Battery"],"prefix":"10.1002","volume":"21","author":[{"given":"Xiaojing","family":"Lin","sequence":"first","affiliation":[{"name":"Fujian Key Laboratory of Polymer Materials, College of Chemistry and Materials Science Fujian Normal University  Fuzhou 350007 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Ziyuan","family":"Wu","sequence":"additional","affiliation":[{"name":"Fujian Key Laboratory of Polymer Materials, College of Chemistry and Materials Science Fujian Normal University  Fuzhou 350007 China"},{"name":"State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter Chinese Academy of Sciences  Fuzhou Fujian 350002 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Cong","family":"Xu","sequence":"additional","affiliation":[{"name":"Fujian Key Laboratory of Polymer Materials, College of Chemistry and Materials Science Fujian Normal University  Fuzhou 350007 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yangyang","family":"Ran","sequence":"additional","affiliation":[{"name":"Fujian Key Laboratory of Polymer Materials, College of Chemistry and Materials Science Fujian Normal University  Fuzhou 350007 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jindan","family":"Zhang","sequence":"additional","affiliation":[{"name":"Fujian Key Laboratory of Polymer Materials, College of Chemistry and Materials Science Fujian Normal University  Fuzhou 350007 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Weihua","family":"Deng","sequence":"additional","affiliation":[{"name":"Fujian Key Laboratory of Polymer Materials, College of Chemistry and Materials Science Fujian Normal University  Fuzhou 350007 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-6016-2587","authenticated-orcid":false,"given":"Shengchang","family":"Xiang","sequence":"additional","affiliation":[{"name":"Fujian Key Laboratory of Polymer Materials, College of Chemistry and Materials Science Fujian Normal University  Fuzhou 350007 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-8931-9880","authenticated-orcid":false,"given":"Zhibin","family":"Cheng","sequence":"additional","affiliation":[{"name":"Fujian Key Laboratory of Polymer Materials, College of Chemistry and Materials Science Fujian Normal University  Fuzhou 350007 China"},{"name":"State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter Chinese Academy of Sciences  Fuzhou Fujian 350002 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-1264-7648","authenticated-orcid":false,"given":"Zhangjing","family":"Zhang","sequence":"additional","affiliation":[{"name":"Fujian Key Laboratory of Polymer Materials, College of Chemistry and Materials Science Fujian Normal University  Fuzhou 350007 China"},{"name":"State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter Chinese Academy of Sciences  Fuzhou Fujian 350002 China"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2025,1,31]]},"reference":[{"key":"e_1_2_7_1_1","doi-asserted-by":"publisher","DOI":"10.1021\/acsnano.3c12522"},{"key":"e_1_2_7_2_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.joule.2017.07.001"},{"key":"e_1_2_7_3_1","doi-asserted-by":"publisher","DOI":"10.1021\/acs.chemrev.3c00167"},{"key":"e_1_2_7_4_1","first-page":"120","volume":"68","author":"Xu Y. 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