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This work proposes a pioneering green technology integrating carbon capture and utilization in lithium silicate materials for lithium\u2010ion batteries to realize \u201cReduction Carbon emission Batteries\u201d. Notably, the study is the first in analyzing the CO\n                    <jats:sub>2<\/jats:sub>\n                    emissions occurring during materials fabrication and highlighting a high\u2010energy\u2010efficiency synthesis method superior to traditional approaches, capable of reducing CO\n                    <jats:sub>2<\/jats:sub>\n                    emissions by more than 85%. Furthermore, the as\u2010synthesized materials exhibit outstanding carbon capture ability by fast and efficient carbonation reactions, where the morphological and crystalline evolution are disclosed. Finally, the extreme stable cycling and fast\u2010charging capabilities of the carbonated lithium silicate anode materials for Lithium Ion Batteries are demonstrated. This innovative interdisciplinary research will inspire the advancement of global green energy.\n                  <\/jats:p>","DOI":"10.1002\/smll.202504905","type":"journal-article","created":{"date-parts":[[2025,8,8]],"date-time":"2025-08-08T09:00:33Z","timestamp":1754643633000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Pioneering Strategy of Circulation of Carbon Capture Toward Lithium\u2010Ion Batteries"],"prefix":"10.1002","volume":"21","author":[{"ORCID":"https:\/\/orcid.org\/0000-0003-0479-0452","authenticated-orcid":false,"given":"Yi\u2010Xiu","family":"Chen","sequence":"first","affiliation":[{"name":"Department of Materials Science and Engineering National Cheng Kung University  Tainan 70001 Taiwan"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Arijit","family":"Mitra","sequence":"additional","affiliation":[{"name":"Department of Materials Science and Engineering National Cheng Kung University  Tainan 70001 Taiwan"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Ching\u2010Yuan","family":"Chen","sequence":"additional","affiliation":[{"name":"Department of Materials Science and Engineering National Cheng Kung University  Tainan 70001 Taiwan"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-3642-4556","authenticated-orcid":false,"given":"Chuan\u2010Pu","family":"Liu","sequence":"additional","affiliation":[{"name":"Department of Materials Science and Engineering National Cheng Kung University  Tainan 70001 Taiwan"},{"name":"Hierarchical Green\u2010Energy Materials (Hi\u2010GEM) Research Center National Cheng Kung University  Tainan 70001 Taiwan"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2025,8,8]]},"reference":[{"key":"e_1_2_8_1_1","doi-asserted-by":"publisher","DOI":"10.1039\/C7EE02342A"},{"key":"e_1_2_8_2_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41560-023-01340-6"},{"key":"e_1_2_8_3_1","doi-asserted-by":"publisher","DOI":"10.1039\/D0EE03382K"},{"key":"e_1_2_8_4_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41560-020-0646-1"},{"key":"e_1_2_8_5_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.pecs.2021.100965"},{"key":"e_1_2_8_6_1","unstructured":"(U.S.) D. o. 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